Abstract:A simulation of the measured coherent excitation profile (CEP) of the resonance coherent anti-Stokes Raman scattering (CARS) of ZnPc in a polymer film is carried out by applying the transform theory, which relates the scattering amplitudes to the recorded absorption spectrum. Since the CEP was recorded by varying only the pump frequency at a fixed Stokes frequency (not scanning both at a fixed difference of pump and Stokes beams as usual), the transform relations could not be applied directly but had to be mod… Show more
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