Miniaturized spectrometers have attracted
much attention
due to
their capability to detect spectral information within a small size.
However, such technology still faces challenges including large-scale
preparation and performance repeatability. In this work, we overcome
these challenges by demonstrating a microspectrometer constructed
with a series of pixelized graded-bandgap perovskite photodetectors
fabricated with inkjet printing. High-quality perovskite films with
minimal pinholes and large grains are deposited by optimizing printing
conditions including substrate temperature and surface modification.
The resulting perovskite photodetectors show decent photosensing performance,
and the different photodetectors based on perovskite films with different
bandgaps exhibit various spectral responsivities with different cutoff
wavelength edges. Microspectrometers are then constructed with the
array of the pixelized graded-bandgap perovskite photodetectors, and
incident spectra are algorithmically reconstructed by combining their
output currents. The reconstruction performance of the miniaturized
spectrometer is evaluated by comparing the results to the spectral
curve measured with a commercial bulky spectrometer, indicating a
reliable spectral reconstruction with a resolution of around 10 nm.
More significantly, the miniaturized spectrometers are successfully
fabricated on polymer substrates, and they demonstrate excellent mechanical
flexibility. Therefore, this work provides a flexible miniaturized
spectrometer with large-scale fabricability, which is promising for
emerging applications including wearable devices, hyperspectral imaging,
and internet of things.