Boosting Reactive Oxygen Species Formation Over Pd and VOδ Co‐Modified TiO2 for Methane Oxidation into Valuable Oxygenates
Huanyu Zhou,
Fan Chen,
Dandan Liu
et al.
Abstract:Direct photocatalytic methane oxidation into value‐added products provides a promising strategy for methane utilization. However, the inefficient generation of reactive oxygen species (ROS) partly limits the activation of CH4. Herein, it is reported that Pd and VOδ co‐modified TiO2 enables direct and selective methane oxidation into liquid oxygenates in the presence of O2 and H2. Due to the extra ROS production from the in situ formed H2O2, a highly improved yield rate of 5014 µmol g−1 h−1 for liquid oxygenate… Show more
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