Boosting Methane Combustion over Pd/Y2O3–ZrO2 Catalyst by Inert Silicate Patches Tuning Both Palladium Chemistry and Support Hydrophobicity
Yang Wu,
Wenhu Yang,
Hailong Zhang
et al.
Abstract:Supported palladium (Pd) catalysts are widely utilized to reduce the emission of exhaust CH 4 from lean-burn engines by catalytic combustion. A large amount of water vapor in the exhaust makes hydroxyls accumulate on the catalyst surface at temperatures below 450 °C, leading to severe catalyst deactivation. Tuning palladium chemistry and inhibiting water adsorption are critical to developing active catalysts. Modifying the support surface with inert silicates would both change the palladium−support interaction… Show more
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