2023
DOI: 10.26434/chemrxiv-2022-09j0v-v2
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Boosting CO2 Photoreduction by π-π-Induced Preassembly between a Cu(I) Photosensitizer and a Pyrene-Appended Co(II) Catalyst

Abstract: The design of a highly efficient system for CO2 photoreduction fully based on earth-abundant elements presents a challenge, which may be overcome by installing suitable interactions between photosensitizer and catalyst to expedite the intermolecular electron transfer. Herein we have designed a pyrene-decorated Cu(I) complex with a rare dual-emission behavior, aiming at additional π-interaction with a pyrene-appended Co(II) catalyst for visible-light-driven CO2-to-CO conversion. The results of 1H NMR titration,… Show more

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