Flexible piezoresistive pressure sensors have promising
applications
in wearable devices, artificial intelligence, and other fields. However,
developing low-cost and high-performance pressure sensors still poses
a great challenge. Herein, we utilize low-cost carbon black (CB) and
multi-walled carbon nanotubes (MWCNTs) mixed in porous polydimethylsiloxane
to assemble a flexible piezoresistive pressure sensor combined with
interdigitated electrodes. Simultaneously, the COMSOL Multiphysics
simulation analysis was performed to predict the sensing behavior
of the pressure sensor, which was verified by experiments; the preparation
of the pressure sensor was guided according to the prediction. Additionally,
we studied the effects of the mixed conductive filler’s weight
ratio, the shape of the interdigital electrode, and the line width
and spacing of the interdigital electrode on the performance of the
sensor. Based on the interaction of the 3D porous structure and the
synergistic conductive network of CB/MWCNTs, the prepared pressure
sensor exhibits a high sensitivity of 3.57 kPa–1 (∼21 kPa), a wide detection range of 0–275 kPa, fast
response time (96 ms), fast recovery time (198 ms), good durability
(about 3000 cycles), and good flexibility. Moreover, the fabricated
sensor can monitor and recognize human activities (such as finger
bending and mouse clicking), indicating that it has great potential
in flexible wearable devices and other fields. It is worth noting
that the preparation process of the entire pressure sensor was simple,
low cost, and environmentally friendly, which provides a certain basis
for industrial and commercial applications.