Bilayer Interphase for Air‐Stable and Dendrite‐Free Lithium Metal Anode Cycling in Carbonate Electrolytes
A‐Re Jeon,
Byeol Yi Han,
Minhyung Kwon
et al.
Abstract:The intrinsic reactivity of lithium (Li) toward ambient air, combined with insufficient cycling stability in conventional electrolytes, hinders the practical adoption of Li metal anodes in rechargeable batteries. Here, a bilayer interphase for Li metal is introduced to address both its susceptibility to corrosion in ambient air and its deterioration during cycling in carbonate electrolytes. Initially, the Li metal anode is coated with a conformal bottom layer of polysiloxane bearing methacrylate, followed by f… Show more
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