We performed the epitaxial growth of the GaN layer on MOCVD-grown GaN templates by plasmaassisted MBE (rf-MBE). We investigated the surface morphology and the growth-mode mechanism, varying the growth condition such as the growth rate and the growth temperature. By reducing the growth rate from 0.5 µm/h to 0.2 µm/h, smooth and flat surface was achieved. The rms surface roughness of 0.2-µm/h-GaN films was smaller than that of MOCVD templates. The cause of smooth surface morphology was the restriction of the spiral growth. Moreover, by changing Ga-flux at 0.2-µm/h growth condition, we found that it was important for smooth surface morphology to grow in stoichiometric condition as well as low growth rate. Especially, rf-MBE has the following advantages: (i) heterojunction interface is sharp, (ii) film thickness can be controlled uniformly, (iii) growth temperature is low. Owing to these specific features, rf-MBE is suitable for the growth of heterostructure films. Since almost nitride devices such as laser diodes (LDs) and high electron mobility transistors (HEMTs) utilize heterostructure films, the advantage of the heteroepitaxial growth in rf-MBE is important to fabricate the nitride wafer for the device application. Moreover, rf-MBE is not needed toxic gases such as NH 3 . The growth without toxic gases leads to the preferred features such as low chamber damage, low background carrier density and low impurity incorporations such as hydrogen and carbons in comparison with MOCVD and GSMBE.However, the quality of the rf-MBE-grown nitride films on sapphire was poor in electrical properties especially. In the case of rf-MBE-grown films, GaN layers grown on sapphire substrates have two kinds of the lattice polarities, which are (0001) Ga-polarity and (000-1) N-polarity. Therefore, the main reason of the poor film-quality is that (0001) Ga-polarity GaN grains and (000-1) N-polarity ones coexist [4].In previous study, we achieved the high-quality rf-MBE-grown GaN films with Ga-polarity by using In exposure and AlN buffer layer [5,6]. Using these Ga-polarity films, AlGaN/GaN HEMTs were fabri-