Bi-functionality of Fe-TUD-1 mesoporous material in Friedel-Crafts' type reactions

Hamdy, Mohamed S.; Mul, Guido; Hamminga, Gerben M.; Moulijn, Jacob A.; Jansen, J.C.

doi:10.1016/s0167-2991(05)80504-x

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Cited by 3 publications

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“…TUD-1 has a 3D mesoporous structure which gives rise to a high accessibility for the substrates. Also TUD-1 can be functionalized with different transition elements [9] such as Ti [10,11], Fe [12,13], and Co [14,15]. The catalytic activity of these materials in various reactions outperformed other mesoporous materials.…”

Section: Introductionmentioning

confidence: 99%

Fe, Co and Cu-incorporated TUD-1: Synthesis, characterization and catalytic performance in N2O decomposition and cyclohexane oxidation

et al. 2005

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Section: Introductionmentioning

confidence: 99%

Fe, Co and Cu-incorporated TUD-1: Synthesis, characterization and catalytic performance in N2O decomposition and cyclohexane oxidation

et al. 2005

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TUD‐1‐Encapsulated HY Zeolite: A New Hierarchical Microporous/Mesoporous Composite with Extraordinary Performance in Benzylation Reactions

Hamdy

Mul

2013

ChemCatChem

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A new composite material consisting of amorphous TUD‐1 encapsulating crystalline zeolite Y was synthesized. Samples with different HY zeolite loadings (10, 20, 40, and 60 wt %) were prepared, and the resulting solid products were characterized with elemental analysis, XRD, N2 physisorption, 27Al MAS NMR, IR, pyridine adsorption in combination with FTIR, temperature‐programmed desorption of ammonia, HRSEM, and HRTEM. Characterization data confirm the presence of a thin layer of the mesoporous TUD‐1 phase with a thickness of 30–100 nm surrounding the zeolite crystals. The catalytic performance of the composite was studied in the Friedel–Crafts benzylation of benzene with benzyl alcohol at 353 K. The catalytic activity of the HY/TUD‐1 composite was higher than that of HY zeolite, whereas the composite showed a much slower rate of deactivation. The improved performance of the composite is related to beneficial changes in the acidity of the HY crystal through chemical interactions with TUD‐1.

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Liquid phase trans-stilbene epoxidation over catalytically active cobalt substituted TUD-1 mesoporous materials (Co-TUD-1) using molecular oxygen

Quek

Tang

et al. 2009

Applied Catalysis A: General

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Bi-functionality of Fe-TUD-1 mesoporous material in Friedel-Crafts' type reactions

Cited by 3 publications

References 15 publications

Fe, Co and Cu-incorporated TUD-1: Synthesis, characterization and catalytic performance in N2O decomposition and cyclohexane oxidation

Fe, Co and Cu-incorporated TUD-1: Synthesis, characterization and catalytic performance in N2O decomposition and cyclohexane oxidation

TUD‐1‐Encapsulated HY Zeolite: A New Hierarchical Microporous/Mesoporous Composite with Extraordinary Performance in Benzylation Reactions

Liquid phase trans-stilbene epoxidation over catalytically active cobalt substituted TUD-1 mesoporous materials (Co-TUD-1) using molecular oxygen

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