“…Because of the giant Rashba spin splitting, the KTO ultrathin lms can be used for achieving circular photogalvanic effect (CPGE) to generate spin-polarized photocurrents. [18][19][20][21][22][23] For the right-handed (le-handed) circularly polarized light, its photon has the angular momentum of +1 (À1), labeled by s + (s À ), and the selection rule for necessary transitions is that the allowed zcomponent change of the total angular momentum is DJ m ¼ +1 (À1). The valence band edge, originating from the J ¼ 3/2 states, has J m ¼ AE3/2, and the conduction band edge, from the Fig.…”