Balancing the Binding of Intermediates Enhances Alkaline Hydrogen Oxidation on D-Band Center Modulated Pd Sites
Yang Zhou,
Chen Tao,
Jiawei Ke
et al.
Abstract:Exploring efficient alkaline hydrogen oxidation reaction
(HOR)
electrocatalysts is of great concern for constructing anion exchange
membrane fuel cells (AEMFCs). Herein, d-band center modulated PdCo
alloys with ultralow Pd content anchored onto the defective carbon
support (abbreviated as PdCo/NC hereafter) are proposed as highly
efficient HOR catalyst. The as-prepared catalyst exhibits exceptional
HOR performance compared to the Pt/C catalyst, achieving thermodynamically
spontaneous and kinetically preferenti… Show more
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