“…For example, the number of spins we can treat is limited to about 24 in the case of an S = 1/2 quantum spin system. For overcoming such the situation, alternative numerical methods without ensemble average [1][2][3][4][5][6] have also been developed and used historically to investigate the thermal nature of the quantum frustrated spin systems, such as triangular [6][7][8][9], kagome [5][6][7][8][10][11][12][13][14][15][16][17], and pyrochlore [18][19][20] magnets. In particular, the method using a typical pure state has got attention recently because it has been proven in different and independent literatures that a single pure state can represent the thermal equilibrium in the thermodynamic limit [2,[4][5][6].…”