“…17 Specifically, CNT fibers comprising of aligned CNT bundles have been attracting great attention owing to their advantageous properties of good electrical conductivity, superior mechanical flexibility, light weight together with satisfactory chemical stability. 12,13,18 Besides, they can be easily tailored with desired properties via engineering their microstructures or incorporating functional material into the fibers, which present broad applications in the field of supercapacitors, [19][20][21] batteries, 22,23 actuators, 2,[24][25][26][27][28] strain sensors, 29,30 etc. To date, flexible fibers with novel functions, such as high stretchability 22,31,32 and self-healing ability, 7 are also highly desirable to withstand the various deformations of bending, twisting, stretching plus the damages during daily usages, thus, satisfying the requirements of practical needs.…”