“…Shape-memory polymers (SMP), one type of smart materials, can deform from the temporary shape to the permanent shape under external stimuli (mainly including heat [12,13], light [14], electric [15], magnetic fields [16], water/solvent [17]), where performance had been programmed before triggering [18,19], and that it has common advantages of polymer: High elastic deformation, low cost, low density, potential biocompatibility, and biodegradability. Indeed, SMP has been widely used in aerospace [20], textile [21], biomedicine [22], kinetic buildings, and other related fields [23]. In order to improving SMP’s physical and chemical properties, one of methods is by introducing filler into polymer matrix, such as wood flour and cellulose whisker [24,25], which all have destroyed the original biological structure and morphology of natural wood.…”