2021
DOI: 10.1021/acsenergylett.1c00939
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Anode for Zinc-Based Batteries: Challenges, Strategies, and Prospects

Abstract: Figure 7. (a) Behavior of bare zinc and Zn|In anodes in an aqueous ZnSO 4 electrolyte and (b) operando optical microscopy images of bare zinc and Zn|In anode in the aqueous ZnSO 4 electrolyte to characterize the gas evolution. Panels a and b reproduced with permission from ref 57.

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Cited by 170 publications
(137 citation statements)
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References 161 publications
(597 reference statements)
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“…[ 6,7 ] However, Zn metal anodes always suffer from side reactions (dendrite growth, H 2 evolution reaction, and corrosion by‐products) in the aqueous electrolytes, significantly hindering their commercialized applications. [ 8–10 ]…”
Section: Introductionmentioning
confidence: 99%
“…[ 6,7 ] However, Zn metal anodes always suffer from side reactions (dendrite growth, H 2 evolution reaction, and corrosion by‐products) in the aqueous electrolytes, significantly hindering their commercialized applications. [ 8–10 ]…”
Section: Introductionmentioning
confidence: 99%
“…Despite the above merits of aqueous Zn-based EES systems, their practical application is hampered by the electrochemical and thermodynamic instability of metallic zinc anodes [18][19][20]. To be specific, during zinc plating/stripping processes, the microscopic surface of zinc anodes changes continuously, thereby causing an inhomogeneous electric field (e.g., protuberance sites generally create a strong localized electrical field due to the "tip effect") [21].…”
Section: Introductionmentioning
confidence: 99%
“…The Zn nucleation tends to proceed in the high Zn 2+ concentration (i.e., high supersaturation) regions, and the Zn atoms will further deposit onto these nuclei, which eventually leads to the formation of “tips” and thus dendrites. [ 24 ] The dendrite formation is largely affected by both the current density and capacity. [ ] Under large current densities, the Zn deposition is significantly accelerated, and the growth of dendrite is promoted.…”
Section: Main Challenges Facing Zn Anodesmentioning
confidence: 99%