Anode–Electrolyte Interface

Wild, Mark

doi:10.1002/9781119297895.ch4

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Lithium–sulfur Battery Technology1

Introduction1

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2023

2024

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Cited by 3 publications

(2 citation statements)

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“…The charging process's basic operation involves many phases. 41 When lithium polysulfides (Li 2 S x ) receive external electrical energy, they undergo oxidation reactions. Lithium ions are released into the electrolyte, and sulphur molecules (S8) are formed as a consequence of this process.…”

Section: Lithium–sulfur Battery Technologymentioning

confidence: 99%

Beyond graphene: exploring the potential of MXene anodes for enhanced lithium–sulfur battery performance

Sandhu,

Imtiaz,

Raza

et al. 2024

RSC Adv.

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Section: Lithium–sulfur Battery Technologymentioning

confidence: 99%

Beyond graphene: exploring the potential of MXene anodes for enhanced lithium–sulfur battery performance

Sandhu,

Imtiaz,

Raza

et al. 2024

RSC Adv.

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“…In addition, many technological challenges, including poor cyclability, low discharging e ciency, and high self-discharge rate, are reported due to the formation of these lithium polysul des [7][8][9]. Alternatively, the use of additives in the electrolyte and implementation of cathode scaffolds to an extent can overcome the problems related to the shuttle phenomenon [10][11][12][13].…”

Section: Introductionmentioning

confidence: 99%

Reaction mechanism of methyl trifluoroacetate (CH3TFA) with lithium polysulfides (Li2S6) in gas and solvent phase

Cheviri,

Lakshmipathi

2023

Theor Chem Acc

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In this DFT study, we have evaluated the reaction mechanism of lithium polysul de (Li 2 S 6 ) with the electrolyte additive methyl tri uoroacetate (CH 3 TFA) in the gas and solvent (dimethoxyethane (DME)) phase at room temperature (298 K) by locating transition states (TS) for the methyl group transfer from CH 3 TFA to Li 2 S 6 , which is reported to produces organosulfur ((CH 3 ) 2 S 6 ). All the reported methyl transfer reactions that lead to the formation of organosulfur are having high barrier energy. The barrier energy difference between gas and solvent phase is maximum of 7 kcal/mol and both the reactions are in extreamely slow regime. therefore, the methyl transfer reaction for the formation of organosulfur implausible at room temperature.

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A first-principles study on chemical adsorption of lithium polysulfide molecules: investigating the influence of carbon, boron, and nitrogen vacancies in boron carbon nitride 2D sheets

Cheviri

Lakshmipathi

2023

Appl. Phys. A

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Anode–Electrolyte Interface

Cited by 3 publications

References 11 publications

Beyond graphene: exploring the potential of MXene anodes for enhanced lithium–sulfur battery performance

Beyond graphene: exploring the potential of MXene anodes for enhanced lithium–sulfur battery performance

Reaction mechanism of methyl trifluoroacetate (CH3TFA) with lithium polysulfides (Li2S6) in gas and solvent phase

A first-principles study on chemical adsorption of lithium polysulfide molecules: investigating the influence of carbon, boron, and nitrogen vacancies in boron carbon nitride 2D sheets

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