The kagome metals AV3Sb5 (A = K, Rb, Cs) under ambient pressure exhibit an unusual charge order, from which superconductivity emerges. In this work, by applying hydrostatic pressure using a liquid pressure medium and carrying out electrical resistance measurements for RbV3Sb5, we find the charge order becomes suppressed under a modest pressure pc (1.4 < pc < 1.6 GPa), while the superconducting transition temperature Tc is maximized. Tc is then gradually weakened with further increase of pressure, before exhibiting another maxima around 22.8 GPa, signifying the presence of a second superconducting dome. Distinct normal state resistance anomalies are found to be associated with the second superconducting dome, similar to KV3Sb5. Our findings point to qualitatively similar temperature-pressure phase diagrams in KV3Sb5 and RbV3Sb5, suggesting a link between the second superconducting dome and the high-pressure resistance anomalies in the AV3Sb5 series.
I. INTRODUCTIONThe kagome metals AV 3 Sb 5 (A = K, Rb, Cs) [1-4] have drawn significant interest recently, with focus on (1) superconductivity with topological surfaces states [2], which raises the prospects of realizing topological superconductivity and Majorana zero modes [5,6]; (2) a large anomalous Hall effect in the absence of local moments [7-9], which possibly results from a charge order that breaks time-reversal symmetry [10,11]; (3) nature of the superconducting pairing, with evidence for nodeless superconducting gaps [12-14], as well as indications for nematic superconductivity [15]; and (4) sensitivity of superconductivity and charge order to pressure-tuning [16][17][18][19][20][21][22][23], likely related to the presence of competing instabilities on the kagome lattice [24][25][26][27][28].With the application of pressure, the charge order becomes quickly suppressed and superconductivity is enhanced, forming a superconducting dome with maximal T c near the pressure at which charge order disappears [16][17][18][19][20][21][22]. While this superconducting dome can be understood to result from the competition between superconductivity and charge order, a second superconducting dome is found in AV 3 Sb 5 at higher pressures [16,[19][20][21][22], whose origin remains unclear. Factors that may be relevant for formation of the second superconducting dome include a pressure-induced Lifshitz transition [20], magnetism suppressing superconductivity in the region between the two superconducting domes [29], reconstruction of the Sb bands due to the formation of interlayer Sb-Sb bonds [30], and a distinct highpressure phase revealed through resistivity anomalies [19]. While two-dome superconductivity is found in all AV 3 Sb 5 materials via resistivity measurements [22], studies of the corresponding normal state from which superconductivity emerges has been limited [19,20]. In particular, it remains unclear whether resistivity anomalies associated with a high-pressure phase in KV 3 Sb 5 [19] is also present in RbV 3 Sb 5 and CsV 3 Sb 5 .In addition, single crystal diffra...