Abstract:Angular-dependences of in-plane and interlayer magnetotransport properties in n-type Bi2Te3 bulk single crystals have been investigated over a broad range of temperatures and magnetic fields. Giant in-plane magnetoresistances (MR) of up to 500% and interlayer MR of up to 200% were observed, respectively. The observed MR exhibits quadratic field dependences in low fields and linear field dependences in high fields. The angular dependences of the MR represent strong anisotropy and twofold oscillations. The obser… Show more
“…Thus, the MR (%) value reduces from 440% to 150% as the temperature is increased from 5 K to 100 K. Moreover, as the field is changed from perpendicular to parallel the MR value reduces to 82% at 5 K under an applied magnetic field of 140 kOe. Further, the same reduces from 82% to 43% as the temperature is increased from 5 K to 100 K. Thus, we get a negligible value of MR in parallel component in comparison to the perpendicular component.Consequently, we can say that the MR is angular dependent [10,11,15]. Figure 5 represents the field derivative MR as a function of magnetic field.…”
We report the angle dependent high field (up to 140 kOe) magneto transport of Bi 2 Te 3 single crystals, a well-known topological insulator. The crystals were grown from melt of constituent elements via solid state reaction route by self-flux method. Details of crystal growth along with their brief characterization up to 5 Tesla applied field was reported by some of us recently [J. Magn. Mag. Mater. 428, 213 (2017)]. The angle dependence of the magneto-resistance (MR) of Bi 2 Te 3 follows the cos () function i.e., MR is responsive, when the applied field is perpendicular (tilt angle = 0 o and/or 180 o ) to the transport current. The low field (±10 kOe) MR showed the signatures of weak anti localization (WAL) character with typical ν-type cusp near origin at 5 K. Further, the MR is linear right up to highest applied field of 140 kOe. The large positive MR are observed up to high temperatures and are above 250% and 150% at 140 kOe in perpendicular fields at 50 K and 100 K respectively. Heat capacity C P (T) measurements revealed the value of Debye temperature (Ѳ D ) to be 135 K. ARPES (angle resolved photoemission spectroscopy) data clearly showed that the bulk Bi 2 Te 3 single crystal consists of a single Dirac cone.
“…Thus, the MR (%) value reduces from 440% to 150% as the temperature is increased from 5 K to 100 K. Moreover, as the field is changed from perpendicular to parallel the MR value reduces to 82% at 5 K under an applied magnetic field of 140 kOe. Further, the same reduces from 82% to 43% as the temperature is increased from 5 K to 100 K. Thus, we get a negligible value of MR in parallel component in comparison to the perpendicular component.Consequently, we can say that the MR is angular dependent [10,11,15]. Figure 5 represents the field derivative MR as a function of magnetic field.…”
We report the angle dependent high field (up to 140 kOe) magneto transport of Bi 2 Te 3 single crystals, a well-known topological insulator. The crystals were grown from melt of constituent elements via solid state reaction route by self-flux method. Details of crystal growth along with their brief characterization up to 5 Tesla applied field was reported by some of us recently [J. Magn. Mag. Mater. 428, 213 (2017)]. The angle dependence of the magneto-resistance (MR) of Bi 2 Te 3 follows the cos () function i.e., MR is responsive, when the applied field is perpendicular (tilt angle = 0 o and/or 180 o ) to the transport current. The low field (±10 kOe) MR showed the signatures of weak anti localization (WAL) character with typical ν-type cusp near origin at 5 K. Further, the MR is linear right up to highest applied field of 140 kOe. The large positive MR are observed up to high temperatures and are above 250% and 150% at 140 kOe in perpendicular fields at 50 K and 100 K respectively. Heat capacity C P (T) measurements revealed the value of Debye temperature (Ѳ D ) to be 135 K. ARPES (angle resolved photoemission spectroscopy) data clearly showed that the bulk Bi 2 Te 3 single crystal consists of a single Dirac cone.
“…Indeed, ARPES experiments [42] Furthermore, the isotropic two-band mode cannot account for the four-fold angle dependence of the resistivity ρ(θ), as delineated in Fig.4(b). Although the surface states of a topological material such as SmB 6 could induce a similar four-fold angular magnetoresistance [61,62], the anisotropy in Fig.4(b) shows that nearly perfect four-fold symmetry should not arise from the crystal surfaces, since the crystal's width (223.33 μm) is much larger than its thickness (138.78 μm). ARPES experiments [42] have revealed that LaSb is topologically trivial.…”
Section: Iii2 Revealing the Bulk Origin Of The Shubnikov -De Haas Omentioning
We report investigations on the magnetotransport in LaSb, which exhibits extremely large magnetoresistance (XMR). Foremost, we demonstrate that the resistivity plateau can be explained without invoking topological protection. We then determine the Fermi surface from Shubnikov -de Haas (SdH) quantum oscillation measurements and find good agreement with the bulk Fermi pockets derived from first principle calculations. Using a semiclassical theory and the experimentally determined Fermi pocket anisotropies, we quantitatively describe the orbital magnetoresistance, including its angle dependence. We show that the origin of XMR in LaSb lies in its high mobility with diminishing Hall effect, where the high mobility leads to a strong magnetic field dependence of the longitudinal magnetoconductance. Unlike a one-band material, when a system has two or more bands (Fermi pockets) with electron and hole carriers, the added conductance arising from the Hall effect is reduced, hence revealing the latent XMR enabled by the longitudinal magnetoconductance. With diminishing Hall effect, the magnetoresistivity is simply the inverse of the longitudinal magnetoconductivity, enabling the differentiation of the electron and hole contributions to the XMR, which varies with the strength and orientation of the magnetic field. This work demonstrates a convenient way to separate the dynamics of the charge carriers and to uncover the origin of XMR in multi-band materials with anisotropic Fermi surfaces. Our approach can be readily applied to other XMR materials.
“…It is also observed that the magnetoresistance in addition to being large is also linear and non-saturating. [17][18][19][20][21][22] Such large and linear magnetoresistance, which does not saturate even at high fields, was first observed in polycrystalline Bismuth and other metals by Kapitza 23,24 and this was explained by Lifshits 25 et al as due to open Fermi surfaces of the metals. However Bismuth has a small and closed Fermi surface.…”
Bi 2 Te 3 is a member of a new class of materials known as topological insulators which are supposed to be insulating in the bulk and conducting on the surface. However experimental verification of the surface states has been difficult in electrical transport measurements due to a conducting bulk. We report low temperature magnetotransport measurements on single crystal samples of Bi 2 Te 3 . We observe metallic character in our samples and large and linear magnetoresistance from 1.5 K to 290 K with prominent Shubnikov-de Haas (SdH) oscillations whose traces persist upto 20 K. Even though our samples are metallic we are able to obtain a Berry phase close to the value of π expected for Dirac fermions of the topological surface states. This indicates that we might have obtained evidence for the topological surface states in metallic single crystals of Bi 2 Te 3 . Other physical quantities obtained from the analysis of the SdH oscillations are also in close agreement with those reported for the topological surface states. The linear magnetoresistance observed in our sample, which is considered as a signature of the Dirac fermions of the surface states, lends further credence to the existence of topological surface states.
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