“…Traditional methods for determining radionuclide concentrations in water require the sampling of a large volume of water, followed by evaporation, to form a concentrated water sample for measurements of gamma activities [15], or to form a dry sample for measurements of alpha and beta activities [16]. Despite the baromembrane (based on reverse osmosis) having been developed to reduce the time and effort spent concentrating radionuclides in water [17] and the range of analytical techniques developed for the determination of radionuclides (e.g., inductively coupled plasma mass spectrometry, laser-induced kinetic phosphorimetry, solid phase extraction, electrochemical approaches), a large volume of water, tedious sample pre-treatment, and stringent conditions are still typically required [1,18]. Empore Caesium Rad Disks [19,20], onsite flow filtration/adsorption [21], and nonwoven fabric cartridge filters impregnated with potassium zinc ferrocyanide [22] have also been employed to monitor radionuclides in aquatic environments.…”
Existing methods for monitoring radionuclides in aquatic environments require frequent sampling of a large volume of water, followed by tedious concentration and analytical procedures, which often make it impractical. Mussels have also been commonly employed to monitor radionuclides but bioaccumulation is significantly affected by physical and biological factors. This study explored the feasibility of using the ‘Artificial Mussel’ (AM) as a new tool for monitoring radionuclides in marine environments. We showed that (a) the uptake and accumulation of 238U, 88Sr, and 133Cs by AMs are directly related to their concentration in water, and equilibrium could be reached within 7 to 8 weeks with high concentration factors. Our results suggest that AMs can serve as an effective and practical tool for monitoring radionuclides in the aquatic environment and overcoming the difficulties faced by existing methods in radionuclide monitoring.
“…Traditional methods for determining radionuclide concentrations in water require the sampling of a large volume of water, followed by evaporation, to form a concentrated water sample for measurements of gamma activities [15], or to form a dry sample for measurements of alpha and beta activities [16]. Despite the baromembrane (based on reverse osmosis) having been developed to reduce the time and effort spent concentrating radionuclides in water [17] and the range of analytical techniques developed for the determination of radionuclides (e.g., inductively coupled plasma mass spectrometry, laser-induced kinetic phosphorimetry, solid phase extraction, electrochemical approaches), a large volume of water, tedious sample pre-treatment, and stringent conditions are still typically required [1,18]. Empore Caesium Rad Disks [19,20], onsite flow filtration/adsorption [21], and nonwoven fabric cartridge filters impregnated with potassium zinc ferrocyanide [22] have also been employed to monitor radionuclides in aquatic environments.…”
Existing methods for monitoring radionuclides in aquatic environments require frequent sampling of a large volume of water, followed by tedious concentration and analytical procedures, which often make it impractical. Mussels have also been commonly employed to monitor radionuclides but bioaccumulation is significantly affected by physical and biological factors. This study explored the feasibility of using the ‘Artificial Mussel’ (AM) as a new tool for monitoring radionuclides in marine environments. We showed that (a) the uptake and accumulation of 238U, 88Sr, and 133Cs by AMs are directly related to their concentration in water, and equilibrium could be reached within 7 to 8 weeks with high concentration factors. Our results suggest that AMs can serve as an effective and practical tool for monitoring radionuclides in the aquatic environment and overcoming the difficulties faced by existing methods in radionuclide monitoring.
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