Abstract:<p>Using ultrafast two-dimensional infrared spectroscopy (2D-IR), a vibrational probe (thiocyanate, SCN<sup>-</sup>) was used to investigate the hydrogen bonding network of a molten salt (ethyl-ammonium nitrate, EAN) compared to that of H2O. The 2D-IR experiments were performed in both parallel () and perpendicular () conditions along with temperature dependence for both EAN (14-130 ˚C) and H2O (5-89 ˚C). With polarization control, the frequency fluctuation correlation function can be separa… Show more
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