In
this work, hydrophobic association physical hydrogels were prepared
by photoinitiated copolymerization of acrylic acid and butyl acrylate,
followed by water immersion. The chemical structure, mechanical properties,
self-healing behavior, and self-recovery properties of the physical
hydrogels were studied in detail. The hydrogel possessed a large number
of carboxyl groups owing to its high content of acrylic acid, and
it was used to adsorb cationic dye. Different from brittle chemical
hydrogels, the as-prepared physical hydrogels exhibited good tolerance
to microwave heating. Thus, the dye-adsorbed hydrogel was successfully
applied for microwave-assisted Fenton degradation of cationic dyes.
Starting from the unique structure and properties of physical hydrogels,
this work successfully explored application scenarios of these systems
in dye adsorption and microwave-assisted degradation. The present
findings will contribute to understand the relationships among structure,
properties, and practical applications of physical hydrogels.