Abstract. Quantitative analysis of the optical conductivity σ(ω) for the normal state of IronBased superconductors CeOFeAs have been made within the two-component scheme: one is the coherent Drude free carrier excitations and other is incoherent motion of carriers leading to a polaron formation, originated from inter and intra layer transitions of charge carriers. The model successfully accounts for the anomalies reported in the optical measurements for metallic state of the superconductors. The frequency dependent relaxation rates are expressed in terms of memory functions and the coherent Drude carriers from the effective interaction potential leads to a sharp peak at zero frequency which is an indication of metallic conduction and a long tail at higher frequencies, i.e. in the infrared region. While to that the hopping of carriers from Fe to Fe in the FeAs layer and from FeAs layer to CeO layer (incoherent motion of carriers) yields two-peak value around 100 cm -1 and 425 cm -1 respectively in the optical conductivity centred at mid-infrared region. Both the Drude and hopping carriers contribute to the optical process of conduction in the iron-based superconductors and shows similar results on optical conductivity in the mid-infrared as well as infrared frequency regions as those revealed from experiments.
IntroductionThe discovery of non-copper-based superconductors has attracted wide attention to elucidate the mechanism of superconductivity and to explore higher T c materials. It is believed that strong electron correlation and layered structures may play an important role. However, the T c of the non-copperbased superconductors is still lower than 40 K as predicted by BCS theory and experimental evidence. Recently, superconductivity in iron and nickel-based layered quaternary compounds has been reported: LaOFeP (T c = 4 K) [1], LaONiP (T c = 3 K) [2], Later on Kamihara et al. [3] found that by substituting P with As, and partially O with F in LaOFeP, the resultant material La(O 1−x F x )FeAs (x=0.05-0.12) became superconductive at 26K. The Fe 2 As 2 layer, which is sandwiched between the La 2 O 2 layers, serves as a carrier conduction path [1, 2] Thus, conduction carriers are twodimensionally confined in the Fe 2 As 2 layer, causing strong interactions among the electrons.Chen et al. has presented the reflectance and conductivity spectra in a far-infrared region for CeOFeAs and LaOFeAs [4]. The reflectance below 400 cm -1 is strongly suppressed at low frequency below the phase transition temperature, which is a strong indication for the formation of an energy gap. However, the low-frequency reflectance still increases fast towards unity at zero frequency, indicating a metallic behavior. Further more, the spin-density wave (SDW) partial gap is observed for