An inter-comparison of tropospheric ozone reanalysis products from CAMS, CAMS-Interim, TCR-1 and TCR-2

Abstract

Abstract. Global tropospheric ozone reanalyses constructed using different state-of-the-art satellite data assimilation systems, prepared as part of the Copernicus Atmosphere Monitoring Service (CAMS-iRean and CAMS-Rean) as well as two fully independent Tropospheric Chemistry Reanalyses (TCR-1 and TCR-2), have been inter-compared and evaluated for the past decade. The updated reanalyses (CAMS-Rean and TCR-2) generally show substantially improved agreements with independent ground and ozonesonde observations over their predecessor versions (CAMS-iRean and TCR-1) for the diurnal, synoptical, seasonal, and decadal variability. The improved performance can be attributed to a mixture of various upgrades, such as revisions in the chemical data assimilation, including the assimilated measurements, and the forecast model performance. The updated chemical reanalyses agree well with each other for most cases, which highlights the usefulness of the current chemical reanalyses in a variety of studies. Meanwhile, significant temporal changes in the reanalysis quality in all the systems can be attributed to discontinuities in the observing systems. To improve the temporal consistency, a careful assessment of changes in the assimilation configuration, such as a detailed assessment of biases between various retrieval products, is needed. Even though the assimilation of multi-species data influences the representation of the trace gases in all the systems and also the precursors’ emissions in the TCR reanalyses, the influence of persistent model errors remains a concern, especially for the lower troposphere. Our comparison suggests that improving the observational constraints, including the continued development of satellite observing systems, together with the optimization of model parameterisations, such as deposition and chemical reactions, will lead to increasingly consistent long-term reanalyses in the future.

Evaluation of tropospheric ozone reanalyses with independent ozonesonde observations in East Asia

“…Moreover, it considers natural and anthropogenic emission sources of 10 chemical compounds (i.e., nitrogen oxides, carbon monoxide) to obtain basic chemical transformation of ozone. For the data assimilation, the Ensemble Kalman filter (EnKF) technique is applied (Hunt et al 2007) using various satellites such as OMI, Tropospheric Emission Spectrometer's (TES), and Measurements of Pollution in the Troposphere (MOPITT).…”

An updated tropospheric chemistry reanalysis and emission estimates, TCR-2, for 2005–2018

“…An exception is the tropics, where the reduced number of ozonesonde observations for the most recent years used in the TCR-2 validation affected the evaluated performance. Huijnen et al (2019) and Christophe et al (2019) compared tropospheric ozone reanalysis products from CAMS, CAMS-Interim, TCR-1 and TCR-2. The updated reanalyses (CAMS-Rean and TCR-2) showed substantially improved agreements with independent ground and ozonesonde observations over their predecessor versions (CAMS-iRean and TCR-1) for the diurnal, synoptical, seasonal, and decadal variability.…”

“…Meanwhile, a strong reanalysis dependence on forecast model performance was found on the near surface concentrations and precursor emissions, associated with insufficient observational constraints (Huijnen et al, 2019;Miyazaki et al, 2020).…”