An experimental simulation of oxygen isotope exchange reaction between amorphous silicate dust and carbon monoxide gas in the early Solar System

Yamamoto, Daiki; Kawasaki, Noriyuki; Tachibana, Shogo; Ishizaki, Lily; Sakurai, Ryosuke; Yurimoto, Hisayoshi

doi:10.1016/j.gca.2024.04.014

Geochimica et Cosmochimica Acta

2024

DOI: 10.1016/j.gca.2024.04.014

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An experimental simulation of oxygen isotope exchange reaction between amorphous silicate dust and carbon monoxide gas in the early Solar System

Daiki Yamamoto,

Noriyuki Kawasaki,

Shogo Tachibana

et al.

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Oxygen Isotope Exchange between Dust Aggregates and Ambient Nebular Gas

Arakawa,

Yamamoto,

Ishizaki

et al. 2024

ApJ

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Meteorites and their components exhibit a diverse range of oxygen isotope compositions, and the isotopic exchange timescale between dust grains and ambient gas is a key parameter for understanding the spatiotemporal evolution of the solar nebula. As dust grains existed as macroscopic aggregates in the solar nebula, it is necessary to consider the isotopic exchange timescales for these aggregates. Here, we theoretically estimate the isotope exchange timescales between dust aggregates and ambient vapor. The isotope exchange process between aggregates and ambient vapor is divided into four processes: (i) supply of gas molecules to the aggregate surface, (ii) diffusion of molecules within the aggregate, (iii) isotope exchange on the surface of constituent particles, and (iv) isotope diffusion within the particles. We evaluate these timescales and assess which one becomes the rate-determining step. We reveal that the isotope exchange timescale is approximately the same as that of the constituent particles when the aggregate radius is smaller than the critical value, which is a few centimeters when considering the exchange reaction between amorphous forsterite aggregates and water vapor.

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Oxygen Isotope Exchange between Dust Aggregates and Ambient Nebular Gas

Arakawa,

Yamamoto,

Ishizaki

et al. 2024

ApJ

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An experimental simulation of oxygen isotope exchange reaction between amorphous silicate dust and carbon monoxide gas in the early Solar System

Cited by 1 publication

References 41 publications

Oxygen Isotope Exchange between Dust Aggregates and Ambient Nebular Gas

Oxygen Isotope Exchange between Dust Aggregates and Ambient Nebular Gas

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