“…We acknowledge discussions with Chuankun Zhang, Christian Sanner and Jun Ye As long as no cw laser source for nuclear clock operation is available, direct frequency comb spectroscopy appears to be the only alternative. Frequency combs in the visible and infrared have been converted into the VUV region via high-harmonic generation (HHG) [16,23,62,71,106,137,154,251,253,271,275,310,324,415,418]. Also, direct frequency-comb spectroscopy of electronic shell transitions has already been performed [71,252,254].…”