This is an open access article under the terms of the Creative Commons Attribution License, which permits use, distribution and reproduction in any medium, provided the original work is properly cited.We review on time and spatially resolved two-color pumpprobe magneto-optical Kerr effect (MOKE) microscopy studies of electron spins in bulk n-GaAs and GaAs (110) quantum wells (QWs) at low lattice temperatures. The influence of photocarrier heating by above-bandgap optical spin excitation on the spatially resolved magneto-optical spin detection is considered in detail. We demonstrate that a continuous-wave (cw) measurement of the local Kerr rotation at a fixed arbitrary probe wavelength in general does not correctly reveal the local spin polarization when hot electrons are present. For bulk GaAs we determine the true lateral electron spin polarization profile from cw measurements of the spatial dependence of the full excitonic Kerr rotation spectrum. For the (110) QWs, we directly obtain the electron spin diffusion coefficient from picosecond real space imaging of the time evolution of an optically excited electron spin packet, which we observe with a spectrally broad probe pulse.
IntroductionSpintronics demands for precise control of the storage, manipulation, and transfer of electron spin coherence in solid state systems [1,2]. In semiconductors, the time and length scales available for these operations are characterized by the spin relaxation time τ s , the spin diffusivity D s , and the related spin mobility μ s [3,4]. Pump-probe MOKE spectroscopy is a particularly valuable tool for the all-optical investigation of spin phenomena in semiconductors and the determination of these parameters. Because of its high temporal and spatial resolution it has been used extensively to study spin relaxation and spin transport in bulk semiconductors and low-dimensional systems [5][6][7][8][9][10][11].Pump-probe MOKE spectroscopy and the related spin noise spectroscopy both infer information on the electron spin system of semiconductors by measuring small changes in the polarization of a linearly polarized probe laser. In spin