Advances in the characterization of inorganic solids using NMR correlation experiments

Rankin, Andrew G. M.; Pourpoint, Frédérique; Duong, Nghia Tuan; Delevoye, Laurent; Amoureux, Jean‐Paul; Lafon, Olivier

doi:10.1016/b978-0-12-823144-9.00192-8

Comprehensive Inorganic Chemistry III 2023

DOI: 10.1016/b978-0-12-823144-9.00192-8

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Advances in the characterization of inorganic solids using NMR correlation experiments

Andrew G. M. Rankin¹,

Frédérique Pourpoint²,

Nghia Tuan Duong³

et al.

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2024

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Cited by 2 publications

References 437 publications

(547 reference statements)

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High-resolution indirect detection of spin-3/2 quadrupolar nuclei in solids using multiple-quantum-filtered through-space D-HMQC experiments

Trébosc,

Lafon,

Amoureux

2024

Solid State Nuclear Magnetic Resonance

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High-resolution indirect detection of spin-3/2 quadrupolar nuclei in solids using multiple-quantum-filtered through-space D-HMQC experiments

Trébosc,

Lafon,

Amoureux

2024

Solid State Nuclear Magnetic Resonance

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Hydrogen in energy and information sciences

Chung,

Cladek,

Hsiau

et al. 2024

MRS Bulletin

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Beyond its fascinating chemistry as the first element in the Periodic Table, hydrogen is of high societal importance in energy technologies and of growing importance in energy-efficient computing. In energy, hydrogen has reemerged as a potential solution to long-term energy storage and as a carbon-free input for materials manufacturing. Its utilization and production rely on the availability of proton-conducting electrolytes and mixed proton–electron conductors for the components in fuel cells and electrolyzers. In computing, proton mediation of electronic properties has garnered attention for electrochemically controlled energy-efficient neuromorphic computing. Incorporation of substitutional and interstitial hydride ions in oxides, though only recently established, enables tuning of electronic and magnetic properties, inviting a range of possible exotic applications. This article addresses common themes in the fundamental science of hydrogen incorporation and transport in oxides as relevant to pressing technological needs. The content covers (1) lattice (or bulk) mechanisms of hydrogen transport, primarily addressing proton transport, but also touching on hydride ion transport; (2) interfacial transport; (3) exploitation of extreme external drivers to achieve unusual response; and (4) advances in methods to probe the hydrogen environment and transport pathway. The snapshot of research activities in the field of hydrogen-laden materials described here underscores exciting recent breakthroughs, remaining open questions, and breathtaking experimental tools now available for unveiling the nature of hydrogen in solid-state matter. Graphical abstract

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Advances in the characterization of inorganic solids using NMR correlation experiments

Cited by 2 publications

References 437 publications

High-resolution indirect detection of spin-3/2 quadrupolar nuclei in solids using multiple-quantum-filtered through-space D-HMQC experiments

High-resolution indirect detection of spin-3/2 quadrupolar nuclei in solids using multiple-quantum-filtered through-space D-HMQC experiments

Hydrogen in energy and information sciences

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