2012
DOI: 10.1103/physrevb.86.064301
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Adiabatic passage with spin locking in Tm3+:YAG

Abstract: In low concentration Tm 3+ :YAG, we observe efficient adiabatic rapid passage (ARP) of thulium nuclear spin over flipping times much longer than T2. Efficient ARP with long flipping time has been observed in monoatomic solids for decades and has been analyzed in terms of spin temperature and of the thermodynamic equilibrium of a coupled spin ensemble. In low-concentration impurity-doped crystals the spin temperature concept may be questioned. A single spin model should be preferred since the impurity ions are … Show more

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Cited by 15 publications
(12 citation statements)
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“…We tried different pump pulse energies from 35 nJ to 360 nJ at both 79 K and 296 K to assess the dependence of phonon lifetime on the number density of excited carriers as mentioned by other authors. 30 In agreement with our previous observations, 24 we could not detect any change as a function of excitation energy. Hence phonon relaxation due to interaction with excited carriers does not appear to play a significant role in our measurements.…”
Section: Data Interpretation and Resultssupporting
confidence: 92%
“…We tried different pump pulse energies from 35 nJ to 360 nJ at both 79 K and 296 K to assess the dependence of phonon lifetime on the number density of excited carriers as mentioned by other authors. 30 In agreement with our previous observations, 24 we could not detect any change as a function of excitation energy. Hence phonon relaxation due to interaction with excited carriers does not appear to play a significant role in our measurements.…”
Section: Data Interpretation and Resultssupporting
confidence: 92%
“…This value of γ is actually close to the one that we expect in the case of spectral diffusion governed by an Ornstein-Uhlenbeck (OU) process [38], for which γ OU = 2/3 [43,44,45]. In this model, the detuning of each spin diffuses in a Markovian fashion within a characteristic time τ c into a Gaussian steady state distribution of spectral width σ, leading to a dephasing rate of ‡ [40]:…”
Section: °Fsupporting
confidence: 73%
“…The non-exponential shape of the efficiency curve shown in figure 4 indicates decoherence due to spectral diffusion [38,39] that might be mitigated by DD techniques [28,29,40,41,42]. To demonstrate that DD can indeed extend the coherence time we performed storage experiments with increasing number of sequences n s = 1, 2, 4, 8 while maintaining n p = 2 (the global number of pulses is then n = 2, 4, 8, 16).…”
Section: °Fmentioning
confidence: 99%
“…This is illustrated in Fig. 3(b) showing similar decay dynamics at two different excitation pulse energies, 57 nJ and 171 nJ, for measurements at 79 K. Consequently, interaction with the excited electrons which 8 was suggested as a coherent phonon relaxation mechanism 23 does not play a significant role in our case.…”
supporting
confidence: 58%