“…In particular, the photocatalytic degradation technology is often used in the treatment of polluted wastewater based on using solar power to activate the photocatalyst, produce reactive oxygen species, change the internal structure of pollutants, and ultimately transform organic pollutants into CO 2 , H 2 O, or other green small molecules that can be naturally degraded. Compared with conventional methods for treating water pollution, the photocatalytic degradation technology exhibits notable advantages, including high efficiency, negligible production of pollution, excellent repeatability, and a straightforward treatment process [9–10] …”
Section: Introductionmentioning
confidence: 99%
“…Compared with conventional methods for treating water pollution, the photocatalytic degradation technology exhibits notable advantages, including high efficiency, negligible production of pollution, excellent repeatability, and a straightforward treatment process. [9][10] The crux of the photocatalysis technology is the development of high-performance photocatalysts. At present, the most commonly used photocatalyst semiconductors are metal oxides [11][12][13] and sulfides; [14] however, these materials can only absorb ultraviolet light in sunlight, causing low efficiency in the photocatalytic degradation of organic pollutants.…”
Graphite carbon nitride (g‐C3N4) has garnered considerable attention due to its excellent photocatalytic properties for the degradation of organic matter in wastewater treatment. Herein, sulfur‐doped g‐C3N4 nanosheets (CN−S‐X) were successfully synthesized via physical steam activation using thiourea and urea as precursors. Comprehensive characterizations demonstrate that the enhanced photocatalysis is attributed to the ultrathin structure, highly active site, vacancy defects, and high specific surface area due to the synergy of S doping and steam activation. The as‐prepared CN−S‐25 photocatalyst exhibits a desirable degradation efficiency of 95.4 % for methylene blue dye with a high degradation rate of 2.65×10−2 min−1 under visible‐light irradiation, which are 2.1 and 5.52 times those for bulk g‐C3N4, respectively as well as good reusability and stability. This study provides a simple and promising strategy to regulate the nanostructure of g‐C3N4 for highly efficient photocatalytic degradation of organic pollutants.
“…In particular, the photocatalytic degradation technology is often used in the treatment of polluted wastewater based on using solar power to activate the photocatalyst, produce reactive oxygen species, change the internal structure of pollutants, and ultimately transform organic pollutants into CO 2 , H 2 O, or other green small molecules that can be naturally degraded. Compared with conventional methods for treating water pollution, the photocatalytic degradation technology exhibits notable advantages, including high efficiency, negligible production of pollution, excellent repeatability, and a straightforward treatment process [9–10] …”
Section: Introductionmentioning
confidence: 99%
“…Compared with conventional methods for treating water pollution, the photocatalytic degradation technology exhibits notable advantages, including high efficiency, negligible production of pollution, excellent repeatability, and a straightforward treatment process. [9][10] The crux of the photocatalysis technology is the development of high-performance photocatalysts. At present, the most commonly used photocatalyst semiconductors are metal oxides [11][12][13] and sulfides; [14] however, these materials can only absorb ultraviolet light in sunlight, causing low efficiency in the photocatalytic degradation of organic pollutants.…”
Graphite carbon nitride (g‐C3N4) has garnered considerable attention due to its excellent photocatalytic properties for the degradation of organic matter in wastewater treatment. Herein, sulfur‐doped g‐C3N4 nanosheets (CN−S‐X) were successfully synthesized via physical steam activation using thiourea and urea as precursors. Comprehensive characterizations demonstrate that the enhanced photocatalysis is attributed to the ultrathin structure, highly active site, vacancy defects, and high specific surface area due to the synergy of S doping and steam activation. The as‐prepared CN−S‐25 photocatalyst exhibits a desirable degradation efficiency of 95.4 % for methylene blue dye with a high degradation rate of 2.65×10−2 min−1 under visible‐light irradiation, which are 2.1 and 5.52 times those for bulk g‐C3N4, respectively as well as good reusability and stability. This study provides a simple and promising strategy to regulate the nanostructure of g‐C3N4 for highly efficient photocatalytic degradation of organic pollutants.
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