Abstract:Hydrogen sulfide is toxic and corrosive gas abundantly
available
in nature. The activation of hydrogen sulfide to produce hydrogen
and elemental sulfur is of great significance for possible applications
in toxic pollutant control and hydrogen energy regeneration. The activation
of H
2
S by transition metal atoms (M = Cr, Mn, and Fe) has
been studied by low-temperature matrix isolation infrared spectroscopy
and quantum chemical calculations. Experimental and theoretical results
indicate t… Show more
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