2015
DOI: 10.1063/1.4934883
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Acoustic phonon spectrum and thermal transport in nanoporous alumina arrays

Abstract: We report results of a combined investigation of thermal conductivity and acoustic phonon spectra in nanoporous alumina membranes with the pore diameter decreasing from D=180 nm to 25 nm. The samples with the hexagonally arranged pores were selected to have the same porosity ≈13%. The Brillouin-Mandelstam spectroscopy measurements revealed bulk-like phonon spectrum in the samples with D=180-nm pores and spectral features, which were attributed to spatial confinement, in the samples with 25-nm and 40-nm pores.… Show more

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Cited by 35 publications
(37 citation statements)
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“…Nevertheless, the full representation of the BLS experiment is the correct approach to yield the elastic and photoelastic parameters of the hPnC constituent components at nanoscale. 28 We have also examined an alternative approach assuming a solidification of F next to the wall. 30 A thin ($10 nm) solidified layer at the interface with low transverse acoustic velocity ($100 m/s) creates few additional features (flat branches) in the band diagram but are not identifiable among the experimental branches.…”
Section: -mentioning
confidence: 99%
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“…Nevertheless, the full representation of the BLS experiment is the correct approach to yield the elastic and photoelastic parameters of the hPnC constituent components at nanoscale. 28 We have also examined an alternative approach assuming a solidification of F next to the wall. 30 A thin ($10 nm) solidified layer at the interface with low transverse acoustic velocity ($100 m/s) creates few additional features (flat branches) in the band diagram but are not identifiable among the experimental branches.…”
Section: -mentioning
confidence: 99%
“…In this work, we use the femtosecond laser 2PP to fabricate square lattice hPnCs based on the zirconium propoxide (ZPO)-based hybrid sol-gel photosensitive material. 26 There are few reports on cavity-type hPnCs with cylindrical nanopores, e.g., with a single crystalline epoxy/air sample, 18 anodic porous alumina containing hexagonal arrays of aligned nanopores oriented normal to the film surface, 27,28 and square arrays of holes of Si-membranes. 29 Using Brillouin light scattering spectroscopy (BLS) in transmission geometry (see Fig.…”
mentioning
confidence: 99%
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“…Details of our BMS measurement procedures have been reported elsewhere. [16][17][18] In order to observe the interference effects, the amplitudes of the interfering spin waves should be approximately the same at the point of observation. The amplitude of the spin wave signal decreases exponentially with the distance from the generating antenna.…”
Section: Brillouin-mandelstam Spectroscopy Measurementsmentioning
confidence: 99%
“…The degree of transport suppression is dictated by the relationship between the characteristic length of the material and the dominant phonon mean free path (MFP) [4]. For example, recent experiments have demonstrated very low thermal conductivities in thin films [5], nanowires [6,7], and porous materials [8][9][10][11][12][13], illustrating the effectiveness of boundary engineering in tuning thermal transport [14].…”
Section: Introductionmentioning
confidence: 99%