2022
DOI: 10.1038/s41565-022-01075-7
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Abrading bulk metal into single atoms

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Cited by 117 publications
(105 citation statements)
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“…In this strategy, the key is the availability and production cost of oxidase-like materials. Although our models for oxidase-like catalysts have their respective limitations on these aspectsnoble metal nanoparticles like Pd–Ag alloys are expensive while the complexity in SAC preparation limits large-scale productionour literature research fortunately revealed quite diverse oxidase-like materials (Table S7), among which some such as TiO 2 /C-QDs catalyst and OA-MnO 2 catalyst may even come at an affordable cost. , In addition, a facile and ecofriendly top-down mechanochemical abrasion method for direct synthesis of single-atom catalyst nanoparticles from bulk metals has been reported recently . Besides, future research efforts may offer us more oxidase-like materials that are easy and cheap to produce on a mass-production scale.…”
Section: Resultsmentioning
confidence: 99%
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“…In this strategy, the key is the availability and production cost of oxidase-like materials. Although our models for oxidase-like catalysts have their respective limitations on these aspectsnoble metal nanoparticles like Pd–Ag alloys are expensive while the complexity in SAC preparation limits large-scale productionour literature research fortunately revealed quite diverse oxidase-like materials (Table S7), among which some such as TiO 2 /C-QDs catalyst and OA-MnO 2 catalyst may even come at an affordable cost. , In addition, a facile and ecofriendly top-down mechanochemical abrasion method for direct synthesis of single-atom catalyst nanoparticles from bulk metals has been reported recently . Besides, future research efforts may offer us more oxidase-like materials that are easy and cheap to produce on a mass-production scale.…”
Section: Resultsmentioning
confidence: 99%
“…84,85 In addition, a facile and ecofriendly top-down mechanochemical abrasion method for direct synthesis of single-atom catalyst nanoparticles from bulk metals has been reported recently. 86 Besides, future research efforts may offer us more oxidase-like materials that are easy and cheap to produce on a mass-production scale.…”
Section: Resultsmentioning
confidence: 99%
“…No acid is required throughout the process, which is environmentally friendly and easy to mass-produce. 81 Metal phthalocyanine material contains natural M–N 4 sites. According to the process of Fig.…”
Section: Preparation Methodsmentioning
confidence: 99%
“…(b and c) M össbauer spectrum and HAADF-STEM image of Fe-SAC. 48 (d) Shockwave method to form thermally stable SACs. 49 (e) Comparison of the shockwave method with other reported methods.…”
Section: Synthesis Methodologies Of Sacsmentioning
confidence: 99%