2019
DOI: 10.26434/chemrxiv.9795338.v1
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A Transient Directing Group Strategy Enables Enantioselective Reductive Heck Hydroarylation of Alkenes

Abstract: Metal-coordinating directing groups have seen extensive use in the field of transition-metal-catalyzed alkene functionalization; however, their waste-generating installation and removal steps limit the efficiency and practicality of reactions that rely on their use. Inspired by developments in asymmetric organocatalysis, where reactions rely on reversible covalent interactions between an organic substrate and a chiral mediator, we have developed a transient-directing-group approach to reductive Heck hydroaryla… Show more

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