A tandem process for in situ H2O2 formation coupled with benzyl alcohol oxidation using Pd–Au bimetallic catalysts

Martinez, Jordan Santiago; Mazarío, Jaime; Gutiérrez‐Tarriño, Silvia; Galdeano-Ruano, Carmen; Gaona-Miguélez, José; Dómine, Marcelo E.; Oña‐Burgos, Pascual

doi:10.1039/d2dt02831j

Dalton Trans.

2022

DOI: 10.1039/d2dt02831j

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A tandem process for in situ H₂O₂ formation coupled with benzyl alcohol oxidation using Pd–Au bimetallic catalysts

Jordan Santiago Martinez

Jaime Mazarío

Silvia Gutiérrez‐Tarriño

et al.

Abstract: Alcohol oxidation is among the most important industrial organic reactions. Traditionally, the best-suited catalysts are Pd, Pt and Au supported nanoparticles. The research community has recently started drawing-up strategies to...

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The Nexus of Innovation: Electrochemically Synthesizing H₂O₂ and Its Integration with Downstream Reactions

Jiang,

Ji,

Zheng

et al. 2023

ACS Mater. Au

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Hydrogen peroxide (H 2 O 2 ) represents a chemically significant oxidant that is prized for its diverse applicability across various industrial domains. Recent innovations have shed light on the electrosynthesis of H 2 O 2 through two-electron oxygen reduction reactions (2e − ORR) or two-electron water oxidation reactions (2e − WOR), processes that underscore the attractive possibility for the on-site production of this indispensable oxidizing agent. However, the translation of these methods into practical utilization within chemical manufacturing industries remains an aspiration rather than a realized goal. This Perspective intends to furnish a comprehensive overview of the latest advancements in the domain of coupled chemical reactions with H 2 O 2 , critically examining emergent strategies that may pave the way for the development of new reaction pathways. These pathways could enable applications that hinge on the availability and reactivity of H 2 O 2 , including, but not limited to the chemical synthesis coupled with H 2 O 2 and waste water treatment byFenton-like reactions. Concurrently, the Perspective acknowledges and elucidates some of the salient challenges and opportunities inherent in the coupling of electrochemically generated H 2 O 2 , thereby providing a scholarly analysis that might guide future research.

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The Nexus of Innovation: Electrochemically Synthesizing H₂O₂ and Its Integration with Downstream Reactions

Jiang,

Ji,

Zheng

et al. 2023

ACS Mater. Au

View full text Add to dashboard Cite

show abstract

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A tandem process for in situ H₂O₂ formation coupled with benzyl alcohol oxidation using Pd–Au bimetallic catalysts

Abstract: Alcohol oxidation is among the most important industrial organic reactions. Traditionally, the best-suited catalysts are Pd, Pt and Au supported nanoparticles. The research community has recently started drawing-up strategies to...

Cited by 1 publication

References 52 publications

The Nexus of Innovation: Electrochemically Synthesizing H₂O₂ and Its Integration with Downstream Reactions

The Nexus of Innovation: Electrochemically Synthesizing H₂O₂ and Its Integration with Downstream Reactions

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A tandem process for in situ H2O2 formation coupled with benzyl alcohol oxidation using Pd–Au bimetallic catalysts

Abstract: Alcohol oxidation is among the most important industrial organic reactions. Traditionally, the best-suited catalysts are Pd, Pt and Au supported nanoparticles. The research community has recently started drawing-up strategies to...

Cited by 1 publication

References 52 publications

The Nexus of Innovation: Electrochemically Synthesizing H2O2 and Its Integration with Downstream Reactions

The Nexus of Innovation: Electrochemically Synthesizing H2O2 and Its Integration with Downstream Reactions

Contact Info

Product

Resources

About

A tandem process for in situ H₂O₂ formation coupled with benzyl alcohol oxidation using Pd–Au bimetallic catalysts

The Nexus of Innovation: Electrochemically Synthesizing H₂O₂ and Its Integration with Downstream Reactions

The Nexus of Innovation: Electrochemically Synthesizing H₂O₂ and Its Integration with Downstream Reactions