2022
DOI: 10.1039/d2tc00785a
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A solution-fabricated tellurium/silicon mixed-dimensional van der Waals heterojunction for self-powered photodetectors

Abstract: Monoelemental two-dimensional (2D) Tellurium (Te) has demonstrated excellent potential candidate for next-generation (opto)electronic devices due to its unique properties such as topological surface states, high carrier mobility, high light absorption...

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Cited by 28 publications
(21 citation statements)
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“…A shift in the transistor threshold voltage could be observed from the upper part of Figure d, indicating that both photoconductive and photogating effects contribute to photocurrent generation . Particularly, the peak R reaches 1.9 × 10 3 A W –1 for near-infrared 980 nm, corresponding to a calculated D of 2.8 × 10 12 Jones (Figure S13 of the Supporting Information), among the highest reported in Te-based photodetectors. , Figure f presents partial time-resolved response curves under 980 nm with a switching frequency of 0.1 and 0.2 Hz for ∼280 continuous cycles, revealing a steady photoresponse characteristic. The full I ph – t spectrum and corresponding response time are shown in Figure S14 of the Supporting Information.…”
Section: Resultsmentioning
confidence: 94%
“…A shift in the transistor threshold voltage could be observed from the upper part of Figure d, indicating that both photoconductive and photogating effects contribute to photocurrent generation . Particularly, the peak R reaches 1.9 × 10 3 A W –1 for near-infrared 980 nm, corresponding to a calculated D of 2.8 × 10 12 Jones (Figure S13 of the Supporting Information), among the highest reported in Te-based photodetectors. , Figure f presents partial time-resolved response curves under 980 nm with a switching frequency of 0.1 and 0.2 Hz for ∼280 continuous cycles, revealing a steady photoresponse characteristic. The full I ph – t spectrum and corresponding response time are shown in Figure S14 of the Supporting Information.…”
Section: Resultsmentioning
confidence: 94%
“…Table 1 compares the device performance with that in the previously reported 2D material‐based photodetectors, implying the superior photovoltaic and photodetection performance of our heterojunction devices. [ 24,30–33 ]…”
Section: Resultsmentioning
confidence: 99%
“…Table 1 compares the device performance with that in the previously reported 2D material-based photodetectors, implying the superior photovoltaic and photodetection performance of our heterojunction devices. [24,[30][31][32][33] Polarization-sensitive photoresponse is a new degree of freedom for extracting the polarization information of light, enabling the photodetection and imaging with higher contrast in a complex environment. [8,34] The prerequisite to realize the polarized light detection is the anisotropic crystal structure and photoabsorption in low-symmetric van der Waals materials such as GeSe, BP, p-Te, ReS 2, and so on.…”
Section: P V Imentioning
confidence: 99%
“…Besides for BP and PdSe 2 , Te has also been used in the development of polarization detectors due to its structural asymmetry, excellent binomial color ratio, and high air stability (42 months). As shown in Figure 8 e, Tao Zheng et al prepared a Te/Si mixed van der Waals heterojunction, which has a large built-in electric field to quickly separate widely-generated carriers and exhibit excellent anisotropy [ 120 ]. Figure 8 f shows photocurrents at different polarization angles, and the photocurrent anisotropy ratio is 2.1 under 635 nm illumination.…”
Section: New Functional Devicementioning
confidence: 99%
“…( d ) Photocurrent of Gr/PdSe 2 /Ge detector as a function of polarization angle at zero bias [ 119 ] (copyright 2019, American Chemical Society). ( e ) Schematic diagram of Te/Si heterojunction detector [ 120 ] (copyright 2022, Royal Society of Chemistry). ( f ) Normalized photocurrent with 635 nm laser at zero bias voltage [ 120 ] (copyright 2022, Royal Society of Chemistry).…”
Section: New Functional Devicementioning
confidence: 99%