Prior to the onset of the ferromagnetic transition in semimetallic EuB6, unusual magnetic and electric behavior have been reported. Using a highly sensitive magneto-optical imaging (MOI) technique, we visualize the behavior of magnetic domains in a EuB6 single crystal. The transformation from a paramagnetic to a ferromagnetic state is shown to be non-Curie Weiss like and proceeds via multiple breaks in the curvature of the temperature-dependent local magnetization. From our experiments, we identify three characteristic boundaries, T * (H), * 1 c T (H) and Tc2(H), in a field -temperature magnetic phase diagram. Using scaling and modified Arrott's plot analysis of isothermal bulk magnetization data, we determine the critical exponents = T and ultimately disappearing at T * . At * 1 cT we observe a significant increase in the spatial inhomogeneity of the local magnetic field distribution associated with the magnetic domain structure disintegrating into smaller magnetized structures. We explain our results via the formation of magnetic polaronic clusters and their coalescing into larger domains.
Introduction:In systems with strong electron correlations, there are transformations from a disordered to an ordered spin configuration. The correlations impact not only their magnetic but also electrical properties significantly. A case in point are rare-earth hexaborides (RB6, R = Ca,