Abstract:Employing high-energy electrode couples and releasing the capacity of anions in the electrolyte are promising avenues to increase the energy density of existing lithium (Li)-based batteries. Herein, we develop a “shuttle-relay” Li metal battery (SRLMB) based on a hybrid Li-rich oxide cathode with graphite as conductive agent and a heteroatom-based gel polymer electrolyte (HGPE). The HGPE was facilely prepared by polymerizing diethyl allyl phosphate (DAP) monomer in-situ in an all-fluorinated electrolyte, which… Show more
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