A multi-scale insight into gas transport in a deep Cenozoic clay

Gonzalez‐Blanco, Laura; Romero, E.

doi:10.1680/jgeot.21.00208

Cited by 5 publications

(3 citation statements)

References 52 publications

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“…In the frame of the WP GAS of EURAD, UPC/ CIMNE geotechnical laboratory studies, for instance, the consequences of the passage of gas in Boom Clay and Opalinus Clay by analysing gas injection tests performed in oedometer cells at constant vertical stress [11,12]. They show that the bedding plane orientation plays a fundamental role in the volume change behaviour during gas migration (Fig.…”

Section: Analysis Of Long-term Gas-related Repository Transientmentioning

confidence: 99%

EURADWASTE’22 Paper – Host rocks and THMC processes in DGR

Levasseur

Sillen

Marschall

et al. 2022

EPJ Nuclear Sci. Technol.

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Deep geological disposal aims to contain and isolate radioactive waste from the biosphere. Repository systems are made of multiple barriers working together, typically comprising the natural geological barrier provided by the repository host rock and its surroundings and an engineered barrier system. Due to their excellent properties for the confinement of contaminants, including low permeability, high sorption capacity, and swelling/self-sealing capacity, clayey materials are considered as engineered and/or natural barriers in most repository designs under development in Europe. During the lifetime of the repository, clay barriers will be exposed to perturbations, among which those are resulting from gas and heat production within the system. It is important to verify that these perturbations will not be detrimental to the good functioning of these barriers. In this paper, it is shown how the two EURAD R&D work packages, GAS and HITEC use a combination of experimental and modelling approaches to increase the understanding and predictability of the impact on clay barriers of the fundamental processes and their couplings related to gas and heat transport respectively, providing building blocks to support the evaluation of the robustness of the repository concepts.

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Section: Analysis Of Long-term Gas-related Repository Transientmentioning

confidence: 99%

EURADWASTE’22 Paper – Host rocks and THMC processes in DGR

Levasseur

Sillen

Marschall

et al. 2022

EPJ Nuclear Sci. Technol.

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show abstract

“…The results indicate that gas transport induced slight expansion of the samples in both orientations, increasing their intrinsic permeability, which suggested the opening of preferential paths. Furthermore, the analyses of the pore network using mercury intrusion porosimetry (MIP) and micro-focus X-ray computed tomography (µ-CT) confirmed the development of gas pathways following the bedding direction or interconnecting bedding planes [4,5].…”

mentioning

confidence: 92%

“…This poorly indurated rock presents sedimentary bedding planes that can act as preferential pathways during the gas invasion. In a previous experimental campaign, samples at two bedding orientations (parallel and orthogonal to the flow) were tested under oedometer conditions [3,4]. The results indicate that gas transport induced slight expansion of the samples in both orientations, increasing their intrinsic permeability, which suggested the opening of preferential paths.…”

mentioning

confidence: 93%

Effectiveness of self-sealing after gas transport in Boom Clay

Gonzalez-Blanco,

Romero,

Levasseur

2023

SEG

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The study of gas transport in low permeable materials is becoming a significant focus in energy-related geotechnics, particularly for managing deep geological disposal of long-lived and heat-emitting radioactive waste. Argillaceous rocks, studied to host the disposal, may present induced fractures caused by the excavation activities that increase the permeability to liquid and gas. The generation of gases can also lead to an excessive pressure build-up in these saturated media resulting in the development or reactivation of fractures/fissures creating preferential pathways for the gas flow [1]. Nevertheless, these rocks present the advantage of self-seal (via swelling of clay minerals due to re-saturation, consolidation or creep), reducing fissure permeability and potentially restoring the barrier function [2]. This study focuses on Boom Clay, a Cenozoic clay candidate for hosting the repository in the Belgian programme, aiming at characterising the effectiveness of its self-sealing process after gas injection/dissipation tests due to the swelling of clay minerals during re-saturation. This poorly indurated rock presents sedimentary bedding planes that can act as preferential pathways during the gas invasion. In a previous experimental campaign, samples at two bedding orientations (parallel and orthogonal to the flow) were tested under oedometer conditions [3, 4]. The results indicate that gas transport induced slight expansion of the samples in both orientations, increasing their intrinsic permeability, which suggested the opening of preferential paths. Furthermore, the analyses of the pore network using mercury intrusion porosimetry (MIP) and micro-focus X-ray computed tomography (µ-CT) confirmed the development of gas pathways following the bedding direction or interconnecting bedding planes [4, 5]. To assess the self-sealing capacity, oedometer tests were carried out at two bedding directions using an oedometer cell with lateral stress measurement to comprehensively understand the stress state and ensure that gas flow occurred through the sample rather than between the sample-ring interface. Prior to the gas injection stage, water permeability was measured. Subsequently, a gas injection/dissipation stage was performed at constant vertical stress. Immediately after, the sample was placed in contact with synthetic water to allow re-saturation. Finally, the water permeability was measured again. The self-sealing capacity of the clay was assessed by comparing the water permeability at both stages. If the obtained values are similar, the barrier function has been restored. Some tests also included a second gas injection to evaluate the potential pathway reopening. MIP and µ-CT data allowed for evaluating microstructural changes due to these processes. The experimental results demonstrate that gas can flow at pressures lower than the minor lateral stress, and the computed effective gas permeability is always higher than the initial intrinsic water permeability, pointing to the opening of preferential pathways (Figure 1a). Water permeability after re-saturation showed values comparable to the initial intrinsic permeability, recovering the hydraulic barrier function thanks to the clay minerals’ swelling (Figure 1a). This indicates the good self-sealing capacity of the Boom Clay. The gas permeability calculated during a second injection/dissipation stage is slightly higher than the initial one, suggesting some memory of the previously opened path (Figure 1a). The self-sealing effect was also observed in the CT images performed under unstressed conditions after water-undrained unloading of the tested samples. The fissures detected after the gas injection (Figure 1b left) are no longer visible after re-saturation within the technique resolution (fissures > 40µm) (Figure 1b middle). However, a small proportion of large and disconnected pores were identified in CT images, likely due to some gas exsolution. Regarding the subsequent gas injection, it again led to the development of fissures following the bedding direction detected with microstructural techniques (Figure 1b right).

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Self-Sealing of Boom Clay After Gas Transport

Gonzalez-Blanco,

Romero,

Levasseur

2023

Rock Mech Rock Eng

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In the geological disposal of high-level radioactive waste in argillaceous rocks, studying the barrier integrity after gas transport and the pathway closure thanks to self-sealing capacity is a crucial aspect for the safety assessment. This paper presents experimental research in Boom Clay (a potential host rock in Belgium) to evaluate the effectiveness of self-sealing and possible fissure reactivation during a second gas invasion event. Initial water permeability under oedometer conditions was first measured on samples at two bedding orientations, being higher the sample with bedding planes parallel to flow, highlighting marked anisotropy. Then, gas injection tests at a constant volume rate were performed. Results indicated that Boom Clay underwent expansion and degradation during gas injection due to the development of fissures that were quantified using microstructural techniques. The computed effective gas permeability was not significantly dependent on bedding orientation and was slightly larger than the initial intrinsic water permeability. The re-saturation of the samples led to a recovery of the initial water permeability for both orientations, replicating the original anisotropy. The microstructural analyses confirmed the gas pathways’ closure, indicating good self-sealing and the regaining of the hydraulic barrier function. However, a small volume of large unconnected pores was detected on undrained unloading before the microstructural study. An additional gas injection after the self-sealing resulted in a higher effective gas permeability and a larger increase in pore volume, suggesting the reopening of fissures generated during the first injection. Finally, the experimental data were compiled within a multi-scale phenomenological model to relate the microstructural information to macroscopic flow transport properties capturing the intrinsic permeability increase on gas invasion and its recovery during self-sealing.

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A multi-scale insight into gas transport in a deep Cenozoic clay

Cited by 5 publications

References 52 publications

EURADWASTE’22 Paper – Host rocks and THMC processes in DGR

EURADWASTE’22 Paper – Host rocks and THMC processes in DGR

Effectiveness of self-sealing after gas transport in Boom Clay

Self-Sealing of Boom Clay After Gas Transport

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