A Li–O2/CO2 battery based on bio-inspired engineering of the Bi2S3/PVP cathode

Gao, Song; Li, Siqi; Han, Miao; E., Yuanlong; Liu, Wanqiang; Jia, Hongsheng; Wang, Fang

doi:10.1039/d4tc00143e

J. Mater. Chem. C

2024

DOI: 10.1039/d4tc00143e

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A Li–O₂/CO₂ battery based on bio-inspired engineering of the Bi₂S₃/PVP cathode

Song Gao,

Siqi Li,

Miao Han

et al.

Abstract: The high overpotential due to the slow kinetics of carbon dioxide reduction (CO2RR) and carbon dioxide evolution (CO2ER) greatly limits the practical application of Li-CO2 batteries. In this paper, PVP/Bi2S3...

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Approaching Splendid Catalysts for Li–CO₂ Battery from the Theory to Practical Designing: A Review

Pan,

Ma,

Wang

et al. 2024

Advanced Materials

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Lithium carbon dioxide (Li–CO2) batteries, noted for their high discharge voltage of approximately 2.8 V and substantial theoretical specific energy of 1876 Wh kg−1, represent a promising avenue for new energy sources and CO2 emission reduction. However, the practical application of these batteries faces significant hurdles, particularly at high current densities and over extended cycle lives, due to their complex reaction mechanisms and slow kinetics. This paper delves into the recent advancements in cathode catalysts for Li–CO2 batteries, with a specific focus on the designing philosophy from composition, geometry, and homogeneity of the catalysts to the proper test conditions and real‐world application. It surveys the possible catalytic mechanisms, giving readers a brief introduction of how the energy is stored and released as well as the critical exploration of the relationship between material properties and performances. Specifically, optimization and standardization of test conditions for Li–CO2 battery research is highlighted to enhance data comparability, which is also critical to facilitate the practical application of Li–CO2 batteries. This review aims to bring up inspiration from previous work to advance the design of more effective and sustainable cathode catalysts, tailored to meet the practical demands of Li–CO2 batteries.

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Approaching Splendid Catalysts for Li–CO₂ Battery from the Theory to Practical Designing: A Review

Pan,

Ma,

Wang

et al. 2024

Advanced Materials

View full text Add to dashboard Cite

show abstract

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A Li–O₂/CO₂ battery based on bio-inspired engineering of the Bi₂S₃/PVP cathode

Abstract: The high overpotential due to the slow kinetics of carbon dioxide reduction (CO2RR) and carbon dioxide evolution (CO2ER) greatly limits the practical application of Li-CO2 batteries. In this paper, PVP/Bi2S3...

Cited by 1 publication

References 38 publications

Approaching Splendid Catalysts for Li–CO₂ Battery from the Theory to Practical Designing: A Review

Approaching Splendid Catalysts for Li–CO₂ Battery from the Theory to Practical Designing: A Review

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A Li–O2/CO2 battery based on bio-inspired engineering of the Bi2S3/PVP cathode

Abstract: The high overpotential due to the slow kinetics of carbon dioxide reduction (CO2RR) and carbon dioxide evolution (CO2ER) greatly limits the practical application of Li-CO2 batteries. In this paper, PVP/Bi2S3...

Cited by 1 publication

References 38 publications

Approaching Splendid Catalysts for Li–CO2 Battery from the Theory to Practical Designing: A Review

Approaching Splendid Catalysts for Li–CO2 Battery from the Theory to Practical Designing: A Review

Contact Info

Product

Resources

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A Li–O₂/CO₂ battery based on bio-inspired engineering of the Bi₂S₃/PVP cathode

Approaching Splendid Catalysts for Li–CO₂ Battery from the Theory to Practical Designing: A Review

Approaching Splendid Catalysts for Li–CO₂ Battery from the Theory to Practical Designing: A Review