“…The flexible actuators are expected to be used as electrical switches for flexible supercapacitor, lithium-ion battery, and other electrochromatic devices. , However, general designs of flexible actuators are based on all-organic or organic/inorganic composite materials, usually subject to slow response, limited lifetime, or high triggering threshold. Ionic electroactive polymer (ionic EAP), electronic EAP, and thermally active polymer are major actuation materials for flexible actuators based on various driving mechanisms. , Most of ionic EAP have low driving voltages (∼several volts), yet their responses are typically slow, in the range of 0.1–10 s. − The response time of thermally active polymers is limited by their low thermal conductivity, as a result usually larger than 0.1 s. − Electronic EAP could respond as fast as down to ∼1 ms, whereas their high driving voltages usually over 1 kV have greatly limited the range of their applications. − Therefore, it is still a great challenge to build flexible actuators, which could rapidly respond to multiple stimuli, with low requirements for driving conditions.…”