Abstract:A molecular-scale electronic device can be built with programmable molecular switches sandwiched between two electrodes. A cyclic disulfide, 1,2-dithiolane, is a promising anchor group for attaching molecules to gold electrodes in such molecular junction devices, since its dithiol-Au linkage (with the disulfide bond broken) can provide added stabilities and reduced current fluctuations. However, operations of the molecular switches under redox conditions might lead to redox processes involving the AuAS bonds a… Show more
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