“…As part of achieving increased dye pick up and enhanced light scattering, multi-layered photoanode architectures involving TiO 2 nanotubes were also introduced. 208,210,211,213,214,216 As mentioned in the case of nanowires and nanorods (Sections 1.8 and 1.9), here also specific functions were assigned to individual layers. In 2014 Wu et al introduced a three-layered photoanode architecture composed of 1D TiO 2 nanotube arrays, 3D TiO 2 microspheres and zero dimensional nanoparticles.…”