A complete ab initio view of Orbach and Raman spin-lattice relaxation in a Dysprosium coordination compound
Matteo Briganti,
Fabio Santanni,
Lorenzo Tesi
et al.
Abstract:The unique electronic and magnetic properties of Lanthanides molecular complexes place them at the forefront of the race towards high-temperature single-ion magnets and magnetic quantum bits. The design of compounds of this class has so far been almost exclusively driven by static crystal field considerations, with emphasis on increasing the magnetic anisotropy barrier. This guideline has now reached its maximum potential and new progress can only come from a deeper understanding of spin-phonon relaxation mech… Show more
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