2013
DOI: 10.1364/oe.21.030693
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A comparative study on chirped-pulse upconversion and direct multichannel MCT detection

Abstract: A comparative study is carried out on two spectroscopic techniques employed to detect ultrafast absorption changes in the mid-infrared spectral range, namely direct multichannel detection via HgCdTe (MCT) photodiode arrays and the newly established technique of chirped-pulse upconversion (CPU). Whereas both methods are meanwhile individually used in a routine manner, we directly juxtapose their applicability in femtosecond pump-probe experiments based on 1 kHz shot-to-shot data acquisition. Additionally, we ex… Show more

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Cited by 16 publications
(17 citation statements)
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“…In previous visible-light-pump and MIR-probe experiments, the bandwidths are narrow [9,28]. In contrast, the bandwidth of our probe pulse is so broad that the entire free-carrier behavior predicted by the Drude model could be experimentally visualized.…”
Section: Resultsmentioning
confidence: 68%
“…In previous visible-light-pump and MIR-probe experiments, the bandwidths are narrow [9,28]. In contrast, the bandwidth of our probe pulse is so broad that the entire free-carrier behavior predicted by the Drude model could be experimentally visualized.…”
Section: Resultsmentioning
confidence: 68%
“…From late 1970's, parametric upconversion is used for time gating application by utilising the fact that the upconversion takes place only when both the pump and the IR fields temporally overlap inside the χ (2) nonlinear medium [209]. This upconversion time gating is primarily explored for studying transient phenomena like fluorescence characterization [210]- [212] and ultrafast time-resolved spectroscopy [54], [124], [165], [213], and been used for detecting objects embedded in scattering media [201], [214] and even for temporal characterization at single-photon level [215], [216]. There are only a few reported results, where time gating is combined with spatial imaging for characterizing transient phenomena of a 2-D object [136], [217].…”
Section: Discussionmentioning
confidence: 99%
“…few mK to K). Researchers have compared the sensitivity of upconversion detectors with direct detectors at different IR operating wavelengths [44], [50]- [54], however, upconversion detectors are still to be optimized for a given application to reach optimal performance.…”
mentioning
confidence: 99%
“…Several groups demonstrated single-shot detection of the MIR supercontinuum by the use of chirped-pulse upconversion (CPU) with solid crystals [8,[18][19][20][21]. Although it is possible to have efficient frequency conversion with solid crystals, the bandwidth of the detection is still limited to ∼600 cm −1 by the phase-matching condition.…”
Section: Chirped Pulse Upconversionmentioning
confidence: 99%