We report a detailed inelastic neutron scattering study of the collective magnetic excitations of overdoped superconducting La 1:78 Sr 0:22 CuO 4 for the energy range 0 -160 meV. Our measurements show that overdoping suppresses the strong response present for optimally doped La 2ÿx Sr x CuO 4 which is peaked near 50 meV. The remaining response is peaked at incommensurate wave vectors for all energies investigated. We observe a strong high-frequency magnetic response for E * 80 meV suggesting that significant antiferromagnetic exchange couplings persist well into the overdoped part of the cuprate phase diagram. DOI: 10.1103/PhysRevLett.99.067002 PACS numbers: 74.72.Dn, 74.25.Ha, 75.40.Gb, 78.70.Nx The occurrence of high-temperature superconductivity is widely believed to be connected to the cuprates' spin degrees of freedom [1]. Thus, we might expect strong spin fluctuations to coexist with superconductivity over the whole superconducting phase diagram. The spin excitations have been well characterized for the insulating antiferromagnetic (AF) [2] and lightly doped [3-6] compositions. For optimally doped compositions, structured excitations have been observed over a wide energy range [7,8]. However, little is known about the high-energy spin dynamics on the overdoped side of the cuprate phase diagram. One of the best materials to investigate this region is single layer La 2ÿx Sr x CuO 4 (LSCO). This system can be doped sufficiently to destroy the superconductive behavior [9], allowing the spin excitations to be studied across the entire superconducting dome. Studying the overdoped part of the phase diagram offers a different view on the emergence of the superconducting state. In contrast to the underdoped regime, superconductivity does not emerge from the ''pseudogap'' state [10]. Rather, it emerges from what appears to be a strongly correlated metallic state [11].In this Letter, we report an inelastic neutron scattering (INS) study of the magnetic response 00 q; ! of an overdoped superconducting sample over a wide energy range (0 -160 meV) and throughout the Brillouin zone. We have chosen the composition La 1:78 Sr 0:22 CuO 4 (T c 26 K), which shows a substantial drop in T c with respect to optimal doping but is nevertheless superconducting (see Fig. 1). We find that the spin excitations are dramatically modified from those observed at optimal doping: The strong peak in the local susceptibility 00 ! present [8] in La 1:84 Sr 0:16 CuO 4 near 50 meV is suppressed, and the remaining response is incommensurate and strongest around E 10 meV and E * 80 meV. Thus, strong spin excitations persist well into the overdoped region of the cuprate phase diagram as required by magnetically mediated models of superconductivity.La 1:78 Sr 0:22 CuO 4 has a tetragonal structure and we use tetragonal indexing to label reciprocal space Q ha ? kb ? lc ? . The magnetic excitations in LSCO are 2D as the strongest magnetic couplings are within the CuO 2 planes. Thus, usually we quote in-plane components of Q. In this notation, the p...