We present Hubble Space Telescope WFC3/IR images of the Cassiopeia A supernova remnant that survey its high-velocity, S-rich debris in the NE jet and SW counterjet regions through [S III] λλ9069, 9531 and [S II] λλ10,287 -10,370 line emissions. We identify nearly 3400 sulfur emitting knots concentrated in ∼120• wide opposing streams, almost triple the number previously known. The vast majority of these ejecta knots lie at projected distances well out ahead of the remnant's forward blast wave and main shell ejecta, extending to angular distance of 320 to the NE and 260 to the SW from the center of expansion. Such angular distances imply undecelerated ejecta knot transverse velocities of 15,600 and 12,700 km s −1 respectively, assuming an explosion date ≈1670 AD and a distance of 3.4 kpc. Optical spectra of knots near the outermost tip of the NE ejecta stream show strong emission lines of S, Ca, and Ar. We estimate a total mass ∼ 0