A Cascade Jet Plasma Oxidation─electroreduction System Using Pd‐Ni Dual‐Site Catalyst for Sustainable Ammonia Production from Air
Jun Ding,
Wenyi Li,
Heng Zhang
et al.
Abstract:Electrocatalytic N2 reduction reaction (eNRR) has been deemed as an alternative approach to the Haber‐Bosch (H‐B) process for ammonia (NH3) production, but it remains a huge challenge. Here jet plasma oxidation of N2 is reported in air into NOx and subsequently NO2− coupling with electrochemical NO2− reduction reaction (pN2─eNO2−RR) over PdNi alloying nanoparticles on N‐doped carbon nanotubes (PdNi/N‐CNTs) for NH3 synthesis. The results demonstrate that the jet plasma reactor possesses excellent gas reforming … Show more
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