3D printing of self-supported solid electrolytes made of glass-derived Li1.5Al0.5Ge1.5P3O12 for all-solid-state lithium-metal batteries

Sabato, A. G.; Eroles, Marc Nuñez; Anelli, Simone; Sierra, Carolina Duque; Gonzalez‐Rosillo, Juan Carlos; Torrell, Marc; Pesce, Arianna; Accardo, Grazia; Casas‐Cabañas, Montse; López-Aranguren, Pedro; Morata, Álex; Tarancón, Albert

doi:10.1039/d3ta01435e

Cited by 9 publications

(3 citation statements)

References 47 publications

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“…For instance, the post- processing in the light-based or as deposition with assisted drying in the AJP has helped with the improved performance. [21,30] Material-wise, a huge effort has been made to adapt common materials and inks to their implementation in printed devices. Due to how driven 3D printing is by sustainability, most of the work in the field has been focused on the use of LFP as cathode material and only high-energy applications have been using NMC and LCO.…”

Section: Discussionmentioning

confidence: 99%

“…However, this is The scoring of each family was done based on the works of references. [4,[14][15][16] [19] Copyright (2018) The Royal Society of only possible with materials that have high thermal stability such as ceramic electrolytes as the ones printed by Sabato et al [21]…”

Section: Light-basedmentioning

confidence: 99%

“…al. where they printed by SLA a 3D Lithium Aluminum Germanium Phosphate (Li 1.5 Al 0.5 Ge 1.5 P 3 O 12 , LAGP) [21] or similar works with DIW, [26] IJP [170] , and SLA templates. [19] Due to the good stability of ceramic electrolytes with Li metal, this type of electrolyte is generally used with Li anode whose surface can adapt well to the pre-printed electrolytes, and the cathode is printed on top of the ceramic.…”

Section: Solid Ceramic Electrolytesmentioning

confidence: 99%

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Materials for 3D Printed Metal and Metal‐Ion Batteries

García Rodríguez,

Medina Santos,

Coelho

et al. 2024

ChemElectroChem

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The review provides an overview of the latest innovations, trends, and challenges in the field of 3D‐printed metal and metal‐ion batteries. It focuses on the materials used in the printing of batteries, including electrodes, electrolytes, and other electroactive components. Compared to other high‐quality reviews on the topic, this review provides a broader selection of materials that are expected to gain attention in the next few years, such as redox‐active polymers and metal‐organic frameworks. This work gives an overview and insight into the latest trends in printing techniques as well as a statistical review of their uses and strengths. We have also gathered the latest works done for each of the material types, and we have taken the opportunity to put them in context and use them to exemplify in which direction is the field going. The review concludes with a critical view of the challenges ahead and a discussion of the direction that the field is taking as well as the external factors that might help to define its future.

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Section: Discussionmentioning

confidence: 99%

Section: Light-basedmentioning

confidence: 99%

Section: Solid Ceramic Electrolytesmentioning

confidence: 99%

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Materials for 3D Printed Metal and Metal‐Ion Batteries

García Rodríguez,

Medina Santos,

Coelho

et al. 2024

ChemElectroChem

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3D Printing Manufacturing of Lithium Batteries: Prospects and Challenges toward Practical Applications

Huo,

Sheng,

et al. 2023

Advanced Materials

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The manufacturing and assembly of components within cells have a direct impact on the sample performance. Conventional processes restrict the shapes, dimensions, and structures of the commercially available batteries. 3D printing, a novel manufacturing process for precision and practicality, is expected to revolutionize the lithium battery industry owing to its advantages of customization, mechanization, and intelligence. This technique can be used to effectively construct intricate 3D structures that enhance the designability, integrity, and electrochemical performance of both liquid‐ and solid‐state lithium batteries. In this study, an overview of the development of 3D printing technologies is provided and their suitability for comparison with conventional printing processes is assessed. Various 3D printing technologies applicable to lithium‐ion batteries have been systematically introduced, especially more practical composite printing technologies. The practicality, limitations, and optimization of 3D printing are discussed dialectically for various battery modules, including electrodes, electrolytes, and functional architectures. In addition, all‐printed batteries are emphatically introduced. Finally, the prospects and challenges of 3D printing in the battery industry are evaluated.

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Additive manufacturing of Proton-Conducting Ceramics by robocasting with integrated laser postprocessing

Pośpiech,

Nadolska,

Cieślik

et al. 2024

Applied Materials Today

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3D printing of self-supported solid electrolytes made of glass-derived Li_1.5Al_0.5Ge_1.5P₃O₁₂ for all-solid-state lithium-metal batteries

Abstract: LAGP solid electrolyte was successfully 3D printed by stereolithography, producing a corrugated shape, which reduced the area specific resistance and improved the durability during cycling.

Cited by 9 publications

References 47 publications

Materials for 3D Printed Metal and Metal‐Ion Batteries

Materials for 3D Printed Metal and Metal‐Ion Batteries

3D Printing Manufacturing of Lithium Batteries: Prospects and Challenges toward Practical Applications

Additive manufacturing of Proton-Conducting Ceramics by robocasting with integrated laser postprocessing

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