3D printed MXene-based films and cellulose nanofiber reinforced hydrogel electrolyte to enable high-performance flexible supercapacitors

Zhou, Guoqiang; Liu, Xinyue; Liu, Chaozheng; Li, Zhenglin; Liu, Chuhang; Shi, Xiaojie; Li, Ziyan; Mei, Changtong; Li, Mei-Chun

doi:10.1039/d3ta06925g

J. Mater. Chem. A

2024

DOI: 10.1039/d3ta06925g

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3D printed MXene-based films and cellulose nanofiber reinforced hydrogel electrolyte to enable high-performance flexible supercapacitors

Guoqiang Zhou,

Xinyue Liu,

Chaozheng Liu

et al.

Abstract: The 3D-printed MXene electrodes hold great promise for the development of next-generation electrochemical devices, offering improved performance, customization, and design flexibility. To this end, it is crucial to improve the...

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Cited by 11 publications

References 61 publications

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3D printing of hydrogels for flexible micro‐supercapacitors

Baig,

Khan,

Ahmad

et al. 2024

FlexMat

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Advances in hydrogel technology have paved the way for novel and valuable capabilities that are being applied to a diverse spectrum of energy storage applications. Hydrogels, originally renowned for their biomedical applications, are now finding translation into the energy storage domain. These versatile materials exhibit promising potential for various energy‐related applications, including but not limited to acting as highly flexible electrolytes, facilitating the development of flexible supercapacitors, and contributing to advancements in energy conversion devices. The tunable properties of hydrogels, their high ion accessibility, and desirable mechanical characteristics position them as promising candidates for enhancing the performance and efficiency of energy storage systems. In this review, we emphasize the integration of hydrogels into flexible micro‐supercapacitors through 3D printing technology, unraveling the charge transport mechanisms inherent in hydrogels. We discuss methods for developing hydrogels with enhanced physicochemical properties, such as improved mechanical strength, flexibility, and charge transport, offering new prospects for next‐generation energy storage devices. With a deeper understanding of gelation chemistry, we showcase significant progress in fabricating stimuli‐responsive, self‐healing, and highly stretchable hydrogels. Furthermore, we present compelling examples highlighting the versatility of hydrogels, including tailorable architectures, conductive nanostructures, 3D frameworks, and multifunctionalities. The application of innovative 3D printing techniques in hydrogel design is poised to yield materials with immense potential in the realm of energy storage.

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3D printing of hydrogels for flexible micro‐supercapacitors

Baig,

Khan,

Ahmad

et al. 2024

FlexMat

View full text Add to dashboard Cite

show abstract

MXene film electrodes with high mechanical strength, graded ion channels and high pseudocapacitive activity enabled by lignin-containing cellulose fibers

Yang,

Li,

Zhang

et al. 2024

International Journal of Biological Macromolecules

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Tough and self-healing all-in-one supercapacitor enabled by triple-network redox carrageenan and sodium carboxymethylcellulose reinforcing gel polymer electrolyte

Zhang,

Liu,

Wang

et al. 2024

Journal of Alloys and Compounds

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3D printed MXene-based films and cellulose nanofiber reinforced hydrogel electrolyte to enable high-performance flexible supercapacitors

Abstract: The 3D-printed MXene electrodes hold great promise for the development of next-generation electrochemical devices, offering improved performance, customization, and design flexibility. To this end, it is crucial to improve the...

Cited by 11 publications

References 61 publications

3D printing of hydrogels for flexible micro‐supercapacitors

3D printing of hydrogels for flexible micro‐supercapacitors

MXene film electrodes with high mechanical strength, graded ion channels and high pseudocapacitive activity enabled by lignin-containing cellulose fibers

Tough and self-healing all-in-one supercapacitor enabled by triple-network redox carrageenan and sodium carboxymethylcellulose reinforcing gel polymer electrolyte

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