“…No clear salt crystals were observed on this 12‐layer structure after 10‐hour continuous operation. The best evaporation rate for the 12‐layer structure reached 2.66 kg m −2 h −1 (see the second red sphere), representing one of the best reported evaporation rates under 1 sun illumination (e.g., 4,11,16 ). When we further pushed the salinity to 10 wt% and performed the same 10‐hour operation, the salt occupancies on the flat and 1‐layer umbrella structures are 64.7% and 12.6%, respectively (as shown in Figure 2C).…”
Section: Resultsmentioning
confidence: 99%
“…Recently, solar‐driven interfacial evaporation received extensive attention due to their potentials in water, energy and environmental sustainability 5–7 . This technique evaporates water from brines or contaminated water using solar thermal effects and is promising to realize zero‐liquid‐discharge (ZLD) desalination 7–11 . In the past decade, researchers developed various advanced materials, 9,12–16 improved thermal management strategies and systems, 8,12,17–20 and cooling technologies 21–23 to improve the overall water productivity.…”
Section: Introductionmentioning
confidence: 99%
“…Salt accumulation on the solar absorber is considered generally undesirable as solar absorbers are mostly black to enable maximum absorption of the sunlight. Formation of salt on the absorber hinders stable vapor generation and gradually deteriorates the solar thermal performance (e.g., 11,31,32 ). Recently, self‐cleaning strategies were proposed to minimize the maintenance requirement for solar vapor generation (e.g., using prewetting, 10 wood, 33–36 and specially designed geometry structures) 9,17,24,26,37–42 .…”
Section: Introductionmentioning
confidence: 99%
“…[5][6][7] This technique evaporates water from brines or contaminated water using solar thermal effects and is promising to realize zero-liquid-discharge (ZLD) desalination. [7][8][9][10][11] In the past decade, researchers developed various advanced materials, 9,[12][13][14][15][16] improved thermal management strategies and systems, 8,12,[17][18][19][20] and cooling technologies [21][22][23] to improve the overall water productivity. Competitions in higher energy conversion efficiency and evaporation rates, 5,9,15,19,24 lower manufacturing costs, 7,[25][26][27] less maintenance requirements, 5,6,9,10,26,28 and multifunctionalization 29,30 are major goals.…”
Desalination of seawater with zero-liquid discharge is a major challenge. Here we developed a three-dimensional "umbrella" architecture to evaporate hypersaline brines of up to 20 wt% using solar-driven interfacial evaporation. By controlling the water pathway and the thickness of the evaporator films to manipulate the salt capacitance of the system, a stable evaporation rate of >2.6 kg m À2 h À1 was achieved over 4-day operation in the laboratory environment with minimized salt accumulation on evaporation surfaces. By placing the system in an outdoor environment with natural wind, the peak evaporation rate was improved to 9.05 kg m À2 h À1 . After a 4-day outdoor test, the total evaporated water by the umbrella system was 3.7Â more than the natural evaporation from a bulk water surface under identical environmental conditions. The predesigned water flow also controlled the local salt accumulation, resulting in easier salt removing and collection, which is highly desired for accelerated salt mining applications.
“…No clear salt crystals were observed on this 12‐layer structure after 10‐hour continuous operation. The best evaporation rate for the 12‐layer structure reached 2.66 kg m −2 h −1 (see the second red sphere), representing one of the best reported evaporation rates under 1 sun illumination (e.g., 4,11,16 ). When we further pushed the salinity to 10 wt% and performed the same 10‐hour operation, the salt occupancies on the flat and 1‐layer umbrella structures are 64.7% and 12.6%, respectively (as shown in Figure 2C).…”
Section: Resultsmentioning
confidence: 99%
“…Recently, solar‐driven interfacial evaporation received extensive attention due to their potentials in water, energy and environmental sustainability 5–7 . This technique evaporates water from brines or contaminated water using solar thermal effects and is promising to realize zero‐liquid‐discharge (ZLD) desalination 7–11 . In the past decade, researchers developed various advanced materials, 9,12–16 improved thermal management strategies and systems, 8,12,17–20 and cooling technologies 21–23 to improve the overall water productivity.…”
Section: Introductionmentioning
confidence: 99%
“…Salt accumulation on the solar absorber is considered generally undesirable as solar absorbers are mostly black to enable maximum absorption of the sunlight. Formation of salt on the absorber hinders stable vapor generation and gradually deteriorates the solar thermal performance (e.g., 11,31,32 ). Recently, self‐cleaning strategies were proposed to minimize the maintenance requirement for solar vapor generation (e.g., using prewetting, 10 wood, 33–36 and specially designed geometry structures) 9,17,24,26,37–42 .…”
Section: Introductionmentioning
confidence: 99%
“…[5][6][7] This technique evaporates water from brines or contaminated water using solar thermal effects and is promising to realize zero-liquid-discharge (ZLD) desalination. [7][8][9][10][11] In the past decade, researchers developed various advanced materials, 9,[12][13][14][15][16] improved thermal management strategies and systems, 8,12,[17][18][19][20] and cooling technologies [21][22][23] to improve the overall water productivity. Competitions in higher energy conversion efficiency and evaporation rates, 5,9,15,19,24 lower manufacturing costs, 7,[25][26][27] less maintenance requirements, 5,6,9,10,26,28 and multifunctionalization 29,30 are major goals.…”
Desalination of seawater with zero-liquid discharge is a major challenge. Here we developed a three-dimensional "umbrella" architecture to evaporate hypersaline brines of up to 20 wt% using solar-driven interfacial evaporation. By controlling the water pathway and the thickness of the evaporator films to manipulate the salt capacitance of the system, a stable evaporation rate of >2.6 kg m À2 h À1 was achieved over 4-day operation in the laboratory environment with minimized salt accumulation on evaporation surfaces. By placing the system in an outdoor environment with natural wind, the peak evaporation rate was improved to 9.05 kg m À2 h À1 . After a 4-day outdoor test, the total evaporated water by the umbrella system was 3.7Â more than the natural evaporation from a bulk water surface under identical environmental conditions. The predesigned water flow also controlled the local salt accumulation, resulting in easier salt removing and collection, which is highly desired for accelerated salt mining applications.
“…The process used a system of self-assembled particles made of an expanded polystyrene (EPS) core and graphene oxide (GO) shell to introduce interfacial solar evaporation that enabled complete water-solute separation. Interfacial solar evaporation has been widely studied in recent years as a sustainable technology with regard to addressing water-energy challenges [ 4 ]. The photothermal, adsorptive, charge, lamellar and multifunctional properties of GO have made it a popular material for potential application in desalination [ 5 , 6 ].…”
Temperature‐sensitive (thermosensitive) hydrogels, which are part of the family of stimulus‐sensitive hydrogels, consist of water‐filled polymer networks that display a temperature‐dependent degree of swelling. Thermosensitive hydrogels, which can undergo phase transition or swell/de‐swell as temperature changes, have great potential in various technological and biomedical purposes for a number of reasons: their temperature response is reversible, hydrogels are stable and easy to prepare, they can be biocompatible and also be suitably combined with other organic and inorganic materials, resulting in new materials with outstanding properties. Among thermosensitive hydrogels poly(N‐isopropylacrylamide) (PNIPAAm) is the most extensively studied because it brings together the best properties of these materials. Consequently, in the past few years, a wide number of applications and new chemical processes to prepare PNIPAAm and their derivatives are being proposed. The objective of this review is to summarize the fundamentals of thermosensitive hydrogels and recent advances in preparation and both technological and biomedical applications of thermosensitive hydrogel, with a special focus on PNIPAAm and their derivatives. Special attention has been given to the discussion of challenges and future research perspectives based on new horizons not yet considered.
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